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arXiv · 2211.05921

Static and dynamic magnetic properties of the spin-5/2 triangle lattice antiferromagnet Na3Fe(PO4)2 studied by 31P NMR

Devi V. Ambika·Qing-Ping Ding·Sebin J. Sebastian·Ramesh Nath·Yuji Furukawa
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Abstract

$^{31}$P nuclear magnetic resonance (NMR) measurements have been carried out to investigate the magnetic properties and spin dynamics of Fe$^{3+}$ ($S$ = 5/2) spins in the two-dimensional triangular lattice (TL) compound Na$_3$Fe(PO$_4$)$_2$. The temperature ($T$) dependence of nuclear spin-lattice relaxation rates ($1/T_1$) shows a clear peak around N\'eel temperature, $T_{\rm N} = 10.9$~K, corresponding to an antiferromagnetic (AFM) transition. From the temparature dependence of NMR shift ($K$) above $T_{\rm N}$, an exchange coupling between Fe$^{3+}$ spins was estimated to be $J/k_{\rm B}\simeq 1.9$~K using the spin-5/2 Heisenberg isotropic-TL model. The temperature dependence of $1/T_1T$ divided by the magnetic susceptibility ($\chi$), $1/T_1T\chi$, above $T_{\rm N}$ proves the AFM nature of spin fluctuations below $\sim$ 50 K in the paramagnetic state. In the magnetically ordered state below $T_{\rm N}$, the characteristic rectangular shape of the NMR spectra is observed, indicative of a commensurate AFM state in its ground state. The strong temperature dependence of 1/$T_1$ in the AFM state is well explained by the two-magnon (Raman) process of the spin waves in a 3D antiferromagnet with a spin-anisotropy energy gap of 5.7 K. The temperature dependence of sublattice magnetization is also well reproduced by the spin waves. Those results indicate that the magnetically ordered state of Na$_3$Fe(PO$_4$)$_2$ is a conventional 3D AFM state, and no obvious spin frustration effects were detected in its ground state.

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Devi V. Ambika, Qing-Ping Ding, Sebin J. Sebastian, Ramesh Nath, Yuji Furukawa. 2022-11-10. Static and dynamic magnetic properties of the spin-5/2 triangle lattice antiferromagnet Na3Fe(PO4)2 studied by 31P NMR. https://doi.org/10.1088/1361-648x%2Fac9e37

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