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arXiv · 2211.16658

Quantum light from lossy semiconductor Rydberg excitons

Valentin Walther·Anders S. Sørensen
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Abstract

The emergence of photonic quantum correlations is typically associated with emitters strongly coupled to a photonic mode. Here, we show that semiconductor Rydberg excitons, which are only weakly coupled to a free-space light mode can produce strongly antibunched fields, i.e. quantum light. This effect is fueled by micron-scale excitation blockade between Rydberg excitons inducing pair-wise polariton scattering events. Photons incident on an exciton resonance are scatted into blue- and red-detuned pairs, which enjoy relative protection from absorption and thus dominate the transmitted light. We demonstrate that this effect persists in the presence of additional phonon coupling, strong non-radiative decay and across a wide range of experimental parameters. Our results pave the way for the observation of quantum statistics from weakly coupled semiconductor excitons.

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Valentin Walther, Anders S. Sørensen. 2022-11-30. Quantum light from lossy semiconductor Rydberg excitons. https://doi.org/10.1103/physrevlett.131.033607

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