Controlled coherent-coupling and dynamics of exciton complexes in a MoSe$_2$ monolayer

Aleksander Rodek; Thilo Hahn; James Howarth; Takashi Taniguchi; Kenji Watanabe; Marek Potemski; Piotr Kossacki; Daniel Wigger; Jacek Kasprzak

arXiv · 2302.13109

Controlled coherent-coupling and dynamics of exciton complexes in a MoSe$_2$ monolayer

Aleksander Rodek·Thilo Hahn·James Howarth·Takashi Taniguchi·Kenji Watanabe·Marek Potemski·Piotr Kossacki·Daniel Wigger·Jacek Kasprzak

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Abstract

Quantifying and controlling the coherent dynamics and couplings of optically active excitations in solids is of paramount importance in fundamental research in condensed matter optics and for their prospective optoelectronic applications in quantum technologies. Here, we perform ultrafast coherent nonlinear spectroscopy of a charge-tunable MoSe$_2$ monolayer. The experiments show that the homogeneous and inhomogeneous line width and the population decay of exciton complexes hosted by this material can be directly tuned by an applied gate bias, which governs the Fermi level and therefore the free carrier density. By performing two-dimensional spectroscopy, we also show that the same bias-tuning approach permits us to control the coherent coupling strength between charged and neutral exciton complexes.

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Aleksander Rodek, Thilo Hahn, James Howarth, Takashi Taniguchi, Kenji Watanabe, Marek Potemski, Piotr Kossacki, Daniel Wigger, Jacek Kasprzak. 2023-02-25. Controlled coherent-coupling and dynamics of exciton complexes in a MoSe$_2$ monolayer. https://arxiv.org/abs/2302.13109

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