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arXiv · 2303.04974

Probing the electronic topological transitions of WTe2 under pressure using ultrafast spectroscopy

Kai Zhang·Fuhai Su·Dayong Liu·Wenjun Wang·Yongsheng Zhang·Zhi Zeng·Zhe Qu·Alexander F. Goncharov
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Abstract

We investigate the nonequilibrium photocarrier dynamics of WTe2 under pressure using the optical pump-probe spectroscopy. The pressure dependences of the electronic relaxation manifest anomalous changes around 0.8, 3.5, and 6 GPa, indicating the abruptions in the electron-phonon interactions. In addition, the coherent phonon oscillations originating from shear mode suddenly disappears above 3.5 GPa, which marks the onset of Td-1T' structural phase transition. Supported by the theoretical calculation, we unveil the electronic topological transitions (ETTs), especially an emergence of a new type-II Weyl point for Td-WTe2 under pressure. Our work demonstrates a novel route to probe the ETTs under pressure.

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Kai Zhang, Fuhai Su, Dayong Liu, Wenjun Wang, Yongsheng Zhang, Zhi Zeng, Zhe Qu, Alexander F. Goncharov. 2023-03-09. Probing the electronic topological transitions of WTe2 under pressure using ultrafast spectroscopy. https://arxiv.org/abs/2303.04974

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