Searcharxiv⌕ Search
Home/Archive/arXiv

arXiv · 2303.14168

Liquid solution centrifugation for safe, scalable, and efficient isotope separation

Joseph F. Wild·Heng Chen·Keyue Liang·Jiayu Liu·Stephen E. Cox·Alex N. Halliday·Yuan Yang
View original source ↗Read source document ↗Export metadata ↓

Abstract

A general method of separating isotopes by centrifuging dissolved chemical compounds in a liquid solution is introduced. This technique can be applied to almost all elements and leads to large separation factors. The method has been demonstrated in several isotopic systems including Ca, Mo, O, and Li with single-stage selectivities of 1.046-1.067 per unit mass difference (e.g., 1.434 in 40Ca/48Ca, 1.134 in 16O/18O), which are beyond the capabilities of various conventional methods of isotope enrichment. Equations are derived to model the process and the results agree with those of the experiments. The scalability of the technique has been demonstrated by performing a three-stage enrichment of 48Ca, and the scalability is more broadly supported through analogies to the gas centrifuge, whereby countercurrent centrifugation can further multiply the separation factor by 5-10 times per stage in a continuous process. Optimal centrifuge conditions and solutions can achieve both high-throughput and highly efficient isotope separation.

Explore related subjects

nucl-exphysics.app-phphysics.chem-ph

Keep this discovery

BibTeXRIS

Joseph F. Wild, Heng Chen, Keyue Liang, Jiayu Liu, Stephen E. Cox, Alex N. Halliday, Yuan Yang. 2023-03-24. Liquid solution centrifugation for safe, scalable, and efficient isotope separation. https://arxiv.org/abs/2303.14168

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

arXiv2026

Reinvestigation of the Yield of the Trinity Device

Previous published analyses of trinitite to determine the yield of the Trinity nuclear explosion used various estimates of the fraction of fission products that became incorporated in trinitite. Furthermore, these studies utilized nuclear data that has subsequently been revised. Utilizing a planar germanium detector, we observed gamma rays produced by the decays of both 137Cs and 239Pu from four samples of trinitite. From the observed 137Cs/239Pu ratios of and a simple analysis method based on current nuclear data and weapons debris studies, we find an average yield of 9.1+-4.5 kilotons from our four samples. While this result is substantially lower than the established total yield of 21 kilotons, it is in reasonable agreement that attributable to fissions in the 239Pu core alone.

nucl-ex↗
arXiv2026

Search for neutrinoless quadruple beta decay of $^{136}$Xe in PandaX-4T detector

The observation of neutrinoless quadruple beta decay (0$\nu$4$\beta$) in the absence of neutrinoless double beta decay (0$\nu$2$\beta$) has been argued to provide a strong indication that neutrinos are Dirac particles. We report a search for 0$\nu$4$\beta$ decay of $^{136}\text{Xe}$ using a total $^{136}\text{Xe}$ exposure of 148.4 kg$\cdot$yr, collected during the commissioning and the first science runs of the PandaX-4T experiment. No significant excess of events over the background is observed. A lower limit on the 0$\nu$4$\beta$ decay half-life of $^{136}\text{Xe}$ is set at 6.01 x $10^{24}$ yr at the 90% confidence level. This result establishes the most stringent constraint on this process in xenon, demonstrating the unique capability of the PandaX-4T detector in probing lepton number violation and shedding light on the fundamental nature of neutrinos.

nucl-ex↗
arXiv2026

Island of Inversion in neutron-rich cobalt isotopes revealed from mass measurements

Mass measurements of the ground and isomeric states of $^{68-70}$Co have been performed using the JYFLTRAP Penning-trap mass spectrometer at the IGISOL facility. The masses were measured, either for the first time for the isomeric states of $^{68}$Co and $^{70}$Co, or with greatly improved precision for the others, removing ambiguities in the mass surface beyond $N=40$. The ordering of the low and high-spin states in $^{68}$Co and $^{70}$Co has also been established. The results, supported by Large-Scale Shell Model and Discrete Non-Orthogonal Shell-Model calculations, show a gradual lowering of intruder states with increasing neutron number, eventually leading to an inversion in $^{70}$Co. These findings clarify previously proposed contradictory interpretations. Finally, we demonstrate the importance of including induced effective 3N forces for a consistent description of binding energies in the island of inversion near $N=40$.

nucl-ex↗