Nonrelativistic and nonmagnetic control of terahertz charge currents via electrical anisotropy in RuO2 and IrO2

Abstract

Precise and ultrafast control over photo-induced charge currents across nanoscale interfaces could lead to important applications in energy harvesting, ultrafast electronics, and coherent terahertz sources. Recent studies have shown that several relativistic mechanisms, including inverse spin-Hall effect, inverse Rashba-Edelstein effect and inverse spin-orbit-torque effect, can convert longitudinally injected spin-polarized currents from magnetic materials to transverse charge currents, thereby harnessing these currents for terahertz generation. However, these mechanisms typically require external magnetic fields and suffer from low spin-polarization rates and low efficiencies of relativistic spin-to-charge conversion. In this work, we present a novel nonrelativistic and nonmagnetic mechanism that directly utilizes the photo-excited high-density charge currents across the interface. We demonstrate that the electrical anisotropy of conductive oxides RuO2 and IrO2 can effectively deflect injected charge currents to the transverse direction, resulting in efficient and broadband terahertz radiation. Importantly, this new mechanism has the potential to offer much higher conversion efficiency compared to previous methods, as conductive materials with large electrical anisotropy are readily available, whereas further increasing the spin-Hall angle of heavy-metal materials would be challenging. Our new findings offer exciting possibilities for directly utilizing these photo-excited high-density currents across metallic interfaces for ultrafast electronics and terahertz spectroscopy.