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arXiv · 2304.08607

Moment canting and domain effects in antiferromagnetic DyRh$_2$Si$_2$

Kristin Kliemt·Michelle Ocker·Sarah Krebber·Susanne Schulz·Denis V. Vyalikh·Cornelius Krellner·Dmitry Yu. Usachov
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Abstract

A combined experimental and theoretical study of the layered antiferromagnetic compound DyRh$_2$Si$_2$ in the ThCr$_2$Si$_2$-type structure is presented. The heat capacity shows two transitions upon cooling, the first one at the N{\'e}el temperature $T_{\rm N}=55\,\rm K$ and a second one at $T_{\rm N2}=12\,\rm K$. Using magnetization measurements, we study the canting process of the Dy moments upon changing the temperature and can assign $T_{\rm N2}$ to the onset of the canting of the magnetic moments towards the $[100]$ direction away from the $c$ axis. Furthermore, we found that the field dependence of the magnetization is highly anisotropic and shows a two-step process for $H\parallel 001$. We used a mean-field model to determine the crystalline electric field as well as the exchange interaction parameters. Our magnetization data together with the calculations reveal a moment orientation close to the $[101]$ direction in the tetragonal structure at low temperatures and fields. Applying photoemission electron microscopy, we explore the (001) surface of the cleaved DyRh$_2$Si$_2$ single crystal and visualize Si- and Dy-terminated surfaces. Our results indicate that the Si-Rh-Si surface protects the deeper lying magnetically active Dy layers and is thus attractive for investigation of magnetic domains and their properties in the large family of LnT$_2$Si$_2$ materials.

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Kristin Kliemt, Michelle Ocker, Sarah Krebber, Susanne Schulz, Denis V. Vyalikh, Cornelius Krellner, Dmitry Yu. Usachov. 2023-04-17. Moment canting and domain effects in antiferromagnetic DyRh$_2$Si$_2$. https://doi.org/10.1103/physrevb.107.224424

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