$\mu^+$ Knight Shift in UTe$_2$: Evidence for Relocalization in a Kondo Lattice

Abstract

The local magnetic susceptibility of the spin-triplet superconductor UTe$_2$ has been investigated by positive muon ($\mu^+$) Knight shift measurements in the normal state. Three distinct $\mu^+$ Knight shift components are observed for a magnetic field applied parallel to the $c$ axis. Two of these exhibit a breakdown in the linear relationship with the bulk magnetic susceptibility ($\chi$) below a temperature $T^* \! \sim \! 30$ K, which points to a gradual emergence of a correlated Kondo liquid. Below $T_{\rm r} \! \sim \! 12$ K linearity is gradually restored, indicating partial relocalization of the Kondo liquid quasiparticles. The third Knight shift component is two orders of magnitude larger, and despite the $c$-axis alignment of the external field, scales with the $a$-axis $\chi$ above $T_{\rm r} \! \sim \! 12$ K. We conjecture that this component is associated with magnetic clusters and the change in the temperature dependence of all three Knight shift components below $T_{\rm r}$ is associated with a change in magnetic correlations. Our findings indicate that prior to the onset of superconductivity the development of the itinerant heavy-electron fluid is halted by a gradual development of local U $5f$-moment fluctuations.