Periodic Atomic Displacements and Visualization of the Electron-Lattice Interaction in the Cuprate

Abstract

Traditionally, X-ray scattering techniques have been used to detect the breaking of the structural symmetry of the lattice, which accompanies a periodic displacement of the atoms associated with charge density wave (CDW) formation in the cuprate pseudogap states. Similarly, the Spectroscopic Imaging Scanning Tunneling Microscopy (SI-STM) has visualized the short-range CDW. However, local coupling of electrons to the lattice in the form of a short-range CDW has been a challenge to visualize, thus a link between these measurements has been missing. Here, we introduce a novel STM-based technique to visualize the local bond length variations obtained from topographic imaging with picometer precision. Application of this technique to the high-Tc cuprate superconductor Bi2Sr2CaCu2O8+{\delta} revealed a high-fidelity local lattice distortion of the BiO lattice as large as 2%. In addition, analysis of local breaking of rotational symmetry associated with the bond lengths reveals modulations around four-unit-cell periodicity in both B1 and E representations in the C4v group of the lattice, which coincides with the uni-directional d-symmetry CDW (dCDW) previously identified within the CuO2 planes, thus providing direct evidence of electron-lattice coupling in the pseudogap state and a link between the X-ray scattering and STM measurements. Overall, our results suggest that the periodic lattice displacements in E representations correspond to a locally-frozen version of the soft phonons identified by the X-ray scattering measurements, and a fluctuation of the bond length is reflected by the fluctuation of the dCDW formation near the quantum critical point.