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arXiv · 2306.02198

Surface Passivation Method for Super-repellence of Aqueous Macromolecular Condensates

Abstract

Solutions of macromolecules can undergo liquid-liquid phase separation to form droplets with ultra-low surface tension. Droplets with such low surface tension wet and spread over common surfaces such as test tubes and microscope slides, complicating \textit{in vitro} experiments. Development of an universal super-repellent surface for macromolecular droplets has remained elusive because their ultra-low surface tension requires low surface energies. Furthermore, nonwetting of droplets containing proteins poses additional challenges because the surface must remain inert to a wide range of chemistries presented by the various amino-acid side-chains at the droplet surface. Here, we present a method to coat microscope slides with a thin transparent hydrogel that exhibits complete dewetting (contact angles $\theta\approx180^\circ)$ and minimal pinning of phase-separated droplets in aqueous solution. The hydrogel is based on a swollen matrix of chemically crosslinked polyethylene glycol diacrylate of molecular weight 12 kDa (PEGDA), and can be prepared with basic chemistry lab equipment. The PEGDA hydrogel is a powerful tool for \textit{in vitro} studies of weak interactions, dynamics, and internal organization of phase-separated droplets in aqueous solutions.

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Andrea Testa, Hendrik T. Spanke, Etienne Jambon-Puillet, Mohammad Yasir, Andreas M. Küffner, Paolo Arosio, Eric R. Dufresne, Robert W. Style, Aleksander A. Rebane. 2023-06-03. Surface Passivation Method for Super-repellence of Aqueous Macromolecular Condensates. https://arxiv.org/abs/2306.02198

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