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arXiv · 2306.10291

Proximity-induced spin-orbit coupling in phosphorene on a WSe$_2$ monolayer

Marko Milivojević·Martin Gmitra·Marcin Kurpas·Ivan Štich·Jaroslav Fabian
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Abstract

We investigate, using first-principles methods and effective-model simulations, the spin-orbit coupling proximity effects in a bilayer heterostructure comprising phosphorene and WSe$_2$ monolayers. We specifically analyze holes in phosphorene around the $\Gamma$ point, at which we find a significant increase of the spin-orbit coupling that can be attributed to the strong hybridization of phosphorene with the WSe$_2$ bands. We also propose an effective spin-orbit model based on the ${\bf C}_{1{\rm v}}$ symmetry of the studied heterostructure. The corresponding spin-orbit field can be divided into two parts: the in-plane field, present due to the broken nonsymmorphic horizontal glide mirror plane symmetry, and the dominant out-of-plane field triggered by breaking the out-of-plane rotational symmetry of the phosphorene monolayer. Furthermore, we also demonstrate that a heterostructure with 60$^\circ$ twist angle exhibits an opposite out-of-plane spin-orbit field, indicating that the coupling can effectively be tuned by twisting. The studied phosphorene/WSe$_2$ bilayer is a prototypical low common-symmetry heterostructure in which the proximity effect can be used to engineer the spin texture of the desired material.

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Marko Milivojević, Martin Gmitra, Marcin Kurpas, Ivan Štich, Jaroslav Fabian. 2023-06-17. Proximity-induced spin-orbit coupling in phosphorene on a WSe$_2$ monolayer. https://doi.org/10.1103/physrevb.108.115311

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