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arXiv · 2306.14198

Imaging lattice reconstruction in homobilayers and heterobilayers of transition metal dichalcogenides

Anna Rupp·Jonas Göser·Zhijie Li·Ismail Bilgin·Anvar Baimuratov·Alexander Högele
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Abstract

Moir\'{e} interference effects have profound impact on the optoelectronic properties of vertical van der Waals structures. Here we establish secondary electron imaging in a scanning electron microscope as a powerful technique for visualizing registry-specific domains in vertical bilayers of transition metal dichalcogenides with common moir\'e phenomena. With optimal parameters for contrast-maximizing imaging of high-symmetry registries, we identify distinct crystal realizations of WSe$_2$ homobilayers and MoSe$_2$-WSe$_2$ heterobilayers synthesized by chemical vapor deposition, and demonstrate ubiquitous lattice reconstruction in stacking-assembled bilayers with near parallel and antiparallel alignment. Our results have immediate implications for the optical properties of registry-specific excitons in layered stacks of transition metal dichalcogenides, and demonstrate the general potential of secondary electron imaging for van der Waals twistronics.

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Anna Rupp, Jonas Göser, Zhijie Li, Ismail Bilgin, Anvar Baimuratov, Alexander Högele. 2023-06-25. Imaging lattice reconstruction in homobilayers and heterobilayers of transition metal dichalcogenides. https://arxiv.org/abs/2306.14198

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