SearcharxivSearch

arXiv · 2310.03082

Exceeding the Chandrasekhar-Clogston limit in flat-band superconductors: A multiband strong-coupling approach

Abstract

Hybrid systems of superconductors and magnets display several intriguing properties, both from a fundamental physics point of view and with practical applications. Promising applications in superconducting spintronics motivate a search for systems where superconductivity can survive larger in-plane critical magnetic fields than the conventional limit. The Chandrasekhar-Clogston (CC) limit applies to thin-film conventional superconductors with in-plane magnetic fields such that orbital effects may be ignored. For a magnetic field strength comparable to the superconducting gap at zero temperature and zero field, a spin-split normal state attains lower free energy than the superconducting state. A multiband superconductor with a flat band placed just below the Fermi surface has been shown to surpass the CC limit using weak-coupling theory. Since the dimensionless coupling determining the critical temperature scales with the density of states, it is natural to anticipate corrections from strong-coupling theory in flat-band systems, owing to the large density of states of the flat bands. We derive Eliashberg equations and the free energy for a multiband superconductor in a magnetic field. First, we show that the CC limit can be exceeded by a small amount in one-band strong-coupling superconductors due to self-energy renormalization of the magnetic field. Next, we consider a two-band system with one flat band and find that the CC limit can be exceeded by a large amount also in strong-coupling theory, even when including hybridization between bands that intersect.

Explore related subjects

Keep this discovery

BibTeXRIS

Kristian Mæland, Asle Sudbø. 2023-10-04. Exceeding the Chandrasekhar-Clogston limit in flat-band superconductors: A multiband strong-coupling approach. https://doi.org/10.1103/physrevb.108.214511

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Out-of-equilibrium relaxation dynamics of the superconducting order parameter in CsV$_3$Sb$_5$

The application of a time-varying strain field drives a superconducting order parameter out of equilibrium. How the order parameter relaxes back to equilibrium depends both on the structure of the superconducting gap and on the nature of quasiparticle scattering. We report the discovery of an ultrasonic attenuation peak inside the superconducting state of the kagome superconductor CsV$_3$Sb$_5$. This peak is the natural consequence of the order parameter relaxation time matching the ultrasonic drive frequency near $T_{\rm c}$. From the measured frequency dependence of the peak, we extract a microscopic scattering time of $\tau_N = 25$ ps. This timescale is two orders of magnitude longer than the elastic scattering time as determined by resistivity measurements, but is comparable to the inelastic scattering time determined by thermal transport. Within the conventional framework of order-parameter relaxation, this implies that elastic scattering is ineffective at relaxing the superconducting condensate, consistent with a sign-preserving $s$-wave state obeying Anderson's theorem.

cond-mat.supr-con

Eight-unit-cell electronic modulations in cuprates originating from local molecular orbitals

The pair density wave (PDW) state with eight-unit-cell (8a0) periodicity has been widely regarded as the primary order in cuprates, yet its existence and origin remain subjects of intense debate. Using spectroscopic imaging scanning tunneling microscopy, we observe spatial modulations of the electronic states with approximately 8a0 periodicity in both the superconducting and insulating regimes of hole-doped Ca2CuO2Cl2 cuprate. We find that the 8a0 spatial patterns are generated by the formation of molecular orbitals by doped holes, which organize into 4a0*4a0 plaquettes as the basic unit. Our results identify the 4a0 molecular orbital as the fundamental electronic building block in cuprates, while the 8a0 PDW represents a spatial subharmonic that emerges at sufficiently high doping.

cond-mat.supr-con

Record-Breaking Elemental Superconductivity in Tetralayer Kagome Borophene

Superconductivity above the liquid-nitrogen temperature remains rare in two-dimensional elemental crystals, where strong covalent bonding often yields high phonon frequencies but insufficient electron-phonon coupling. Here, using first-principles calculations and fully anisotropic Migdal-Eliashberg theory, we predict tetralayer kagome borophene (TKB) stabilized by ABAB covalent stacking, as a liquid-nitrogen-temperature elemental superconductor. With a predicted critical temperature of 102 K, TKB sets a record-high value among previously reported elemental superconductors. Unlike known high-Tc boron-based superconductors dominated by in-plane sigma-bonding states and high-frequency in-plane B-B stretching modes, TKB realizes an out-of-plane s-pz-bonding-mediated pairing mechanism, in which interlayer s-pz bonding states at the Fermi level are strongly coupled to low-frequency out-of-plane vibrations of boron atoms. These results reveal a distinct out-of-plane pairing channel in multilayer borophene and establish covalent stacking engineering as a potential route for high-Tc superconductivity in two-dimensional materials.

cond-mat.supr-con