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arXiv · 2311.03027

Interplay of crystal symmetries and light's topology in high harmonic spectroscopy

Ana García-Cabrera·Roberto Boyero-García·Óscar Zurrón-Cifuentes·Javier Serrano·Julio San Román·Luis Plaja·Carlos Hernández-García
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Abstract

Structured ultrafast laser beams offer unique opportunities to explore the interplay of the angular momentum of light with matter at the femtosecond scale. Linearly polarized vector beams are paradigmatic examples of structured beams whose topology is characterized by a well-defined Poincar\'e index. It has been demonstrated that the Poincar\'e index is a topological invariant during high-order harmonic generation from isotropic targets, such as noble gases. As a result, harmonics are produced as extreme-ultraviolet vector beams, with the same topology as the driver. We demonstrate that this simple conservation rule does not apply to crystalline solids, characterized by their anisotropic non-linear response to the driving excitation. In this context, we identify the topological properties of the harmonic field as unique probes, sensitive to both the microscopic and macroscopic features of the target's complex non-linear response. Our simulations, performed in single-layer graphene but extendable to other solid targets, show that the harmonic field is split into a multi-beam structure whose topology -- different from that of the driver -- encodes information about laser-driven electronic dynamics. Our work opens the route towards using the topological analysis of the high-order harmonic field as a novel spectroscopic tool to reveal the coupling of light and target symmetries in the non-linear response of matter.

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Ana García-Cabrera, Roberto Boyero-García, Óscar Zurrón-Cifuentes, Javier Serrano, Julio San Román, Luis Plaja, Carlos Hernández-García. 2023-11-06. Interplay of crystal symmetries and light's topology in high harmonic spectroscopy. https://arxiv.org/abs/2311.03027

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