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arXiv · 2403.06022

Intrinsic magnetism in KTaO$_3$ heterostructures

Patrick W. Krantz·Alexander Tyner·Pallab Goswami·Venkat Chandrasekhar
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Abstract

There has been intense recent interest in the two-dimensional electron gases (2DEGs) that form at the surfaces and interfaces of KTaO$_3$ (KTO), with the discovery of superconductivity at temperatures significantly higher than those of similar 2DEGs based on SrTiO$_3$ (STO). Like STO heterostructures, these KTO 2DEGs are formed by depositing an overlayer on top of appropriately prepared KTO surfaces. Some of these overlayers are magnetic, and the resulting 2DEGs show signatures of this magnetism, including hysteresis in the magnetoresistance (MR). Here we show that KTO 2DEGs fabricated by depositing AlO$_x$ on top of KTO also show hysteretic MR, indicative of long range magnetic order, even though the samples nominally contain no intrinsic magnetic elements. The hysteresis appears in both the transverse and longitudinal resistance in magnetic fields both perpendicular to and in the plane of the 2DEG. The hysteretic MR has different characteristic fields and shapes for surfaces of different crystal orientations, and vanishes above a few Kelvin. Density functional theory (DFT) calculations indicate that the magnetism likely arises from Ta$^{4+}$ local moments created in the presence of oxygen vacancies.

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Patrick W. Krantz, Alexander Tyner, Pallab Goswami, Venkat Chandrasekhar. 2024-03-09. Intrinsic magnetism in KTaO$_3$ heterostructures. https://doi.org/10.1063/5.0189956

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