SearcharxivSearch

arXiv · 2408.08613

Acceleration and twisting of neutral atoms by strong elliptically polarized short-wavelength laser pulses

Abstract

We have investigated non-dipole effects in the interaction of a hydrogen atom with elliptically polarized laser pulses of intensity 10$^{14}$ W/cm$^2$ with about 8 fs duration. The study was performed within the framework of a hybrid quantum-quasiclassical approach in which the time-dependent Schr\"odinger equation for an electron and the classical Hamilton equations for the center-of-mass (CM) of an atom are simultaneously integrated. It is shown that the spatial inhomogeneity $ \mathbf{k}\cdot\mathbf{r}$ of the laser field and the presence of a magnetic component in it lead to the non-separability of the CM and electron variables in a neutral atom and, as a consequence, to its acceleration. We have established a strict correlation between the total probability of excitation and ionization of an atom and the velocity of its CM acquired as a result of interaction with a laser pulse. The acceleration of the atom weakly depends on the polarization of the laser in the considered region (\mbox{5 eV $\lesssim \hbar\omega \lesssim $ 27 eV}) of its frequencies. However, the transition from linear to elliptical laser polarization leads to the twisting of the atom relative to the axis directed along the pulse propagation (coinciding with the direction of the momentum of the accelerated atom). It is shown that with increasing ellipticity the twisting effect increases and reaches its maximum value with circular polarization. At this point the projection of the orbital angular momentum acquired by the electron onto the direction of the pulse propagation reaches its maximum value. Further exploration of the possibilities for producing accelerated and twisted atoms with electromagnetic pulses is of interest for a number of prospective applications.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Vladimir S. Melezhik, Sara Shadmehri. 2024-08-16. Acceleration and twisting of neutral atoms by strong elliptically polarized short-wavelength laser pulses. https://doi.org/10.1063/5.0263618

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Delay-engineered dynamical phases in a programmable non-Markovian spin oscillator

Non-Markovian dynamics offer a new route towards engineering non-equilibrium matter, where memory and feedback act as programmable resources for controlling order in time. Here we report the realization of a non-Markovian spin oscillator in a hot vapour $^{129}$Xe-Cs co-magnetometer with programmable feedback delay and gain. By tuning these parameters, we observe a hierarchy of dynamical phases, including time-crystalline response, nonlinear bifurcations, and frequency-comb formation. The measured spectra and phase boundaries are captured by linear stability analysis of delayed Bloch equations, revealing these phenomena as different manifestations of the same memory-induced instability structure. These results establish time-delayed feedback as a powerful strategy for controlling non-equilibrium phases, enabling quantum sensing, frequency referencing, and synchronization within a single spin-based platform.

physics.atom-ph

Non-stick vacuum wall collisions with a laser-coolable molecule

Molecular species that are suitable for direct laser cooling are typically considered lost or destroyed if they collide with an ambient temperature vacuum wall. Here, we study surface collisions with aluminum monofluoride (AlF), a laser-coolable molecule that survives this process with unusually high probability. We detect the outgoing AlF molecules from a single wall collision via Doppler-sensitive laser-induced fluorescence spectroscopy, using incoming supersonic (pulsed) and thermochemical (continuous) molecular beams. The angular, velocity and rovibrational level distributions of the outgoing molecules show near-complete thermalisation to the wall in a single collision event. We determine an upper limit to the surface residence time of about 5$~\mu$s, and by monitoring the decay in density of pulses of molecules loaded into a small storage volume, we deduce the surface sticking probability for different materials. For a siloxane-coated metallic surface, the sticking probability of AlF is about 0.015, allowing us to accumulate molecules from the thermochemical source into an ambient temperature storage vessel at densities near $10^{8}~$cm$^{-3}$. This provides a route to compact, portable traps for neutral molecules.

physics.atom-ph

Kinetic modeling of molecular beam formation in a cryogenic buffer-gas cell

Cryogenic buffer-gas cells are widely used to produce cold molecular beams, but the microscopic dynamics governing beam formation remain challenging to model. Here we present fully kinetic simulations of a cryogenic buffer-gas cell using the Direct Simulation Monte Carlo method implemented in the PICLas framework, treating the buffer gas and ablated molecules within a single unified model. We capture characteristic features of cryogenic buffer-gas sources, including plume cooling, directed transport toward the aperture, and the formation of a slow molecular beam, while also resolving energy transfer from the hot ablation plume to the helium buffer gas that is inaccessible to existing approaches relying on the background-gas approximation. Our results demonstrate that fully kinetic simulations can provide detailed insights into buffer-gas cell dynamics and open a route toward a systematic optimization of such sources.

physics.atom-ph