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arXiv · 2409.03565

Surface Magnetism in Fe$_3$GeTe$_2$ Crystals

T. A. Tyson·S. Amarasinghe·AM M. Abeykoon·R. Lalancette·S. K. Du·X. Fang·S. -W. Cheong·A. Al-Mahboob·J. T. Sadowski
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Abstract

The surface magnetization of Fe$_3$GeTe$_2$ was examined by low-energy electron microscopy (LEEM) using an off-normal incidence electron beam. We found that the 180$^o$ domain walls are of Bloch type. Temperature-dependent LEEM measurements yield a surface magnetization with a surface critical exponent $\beta$1 = 0.79 +/- 0.02. This result is consistent with surface magnetism in the 3D semi-infinite Heisenberg ($\beta$1 = 0.84 +/- 0.01) or Ising ($\beta$1 = 0.78 +/- 0.02) models, which is distinctly different from the bulk exponent ($\beta$ = 0.34 +/- 0.07). The measurements reveal the power of LEEM with a tilted beam to determine magnetic domain structure in quantum materials. Single crystal diffraction measurements reveal inversion symmetry-breaking weak peaks and yield space group P-6m2. This Fe site defect-derived loss of inversion symmetry enables the formation of skyrmions in this Fe$_3$GeTe$_2$ crystal.

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T. A. Tyson, S. Amarasinghe, AM M. Abeykoon, R. Lalancette, S. K. Du, X. Fang, S. -W. Cheong, A. Al-Mahboob, J. T. Sadowski. 2024-09-05. Surface Magnetism in Fe$_3$GeTe$_2$ Crystals. https://arxiv.org/abs/2409.03565

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