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arXiv · 2409.19489

Achieving 5 % $^{13}$C nuclear spin hyperpolarization in high-purity diamond at room temperature and low field

Vladimir V. Kavtanyuk·Changjae Lee·Keunhong Jeong·Jeong Hyun Shim
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Abstract

Optically polarizable nitrogen-vacancy (NV) center in diamond enables the hyperpolarization of $^{13}$C nuclear spins at low magnetic field and room temperature. However, achieving a high level of polarization comparable to conventional dynamic nuclear polarization has remained challenging. Here we demonstrate that, at below 10 mT, a $^{13}$C polarization of 5 % can be obtained, equivalent to an enhancement ratio over $7 \times 10^6$. We used high-purity diamond with a low initial nitrogen concentration ($<$ 1 ppm), which also results in a long storage time exceeding 100 minutes. By aligning the magnetic field along [100], the number of NV spins participating in polarization transfer increases fourfold. We conducted a comprehensive optimization of field intensity and microwave (MW) frequency-sweep parameters for this field orientation. The optimum MW sweep width suggests that polarization transfer occurs primarily to bulk $^{13}$C spins through the integrated solid effect followed by nuclear spin diffusion.

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Vladimir V. Kavtanyuk, Changjae Lee, Keunhong Jeong, Jeong Hyun Shim. 2024-09-29. Achieving 5 % $^{13}$C nuclear spin hyperpolarization in high-purity diamond at room temperature and low field. https://arxiv.org/abs/2409.19489

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