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arXiv · 2501.19230

Electron-beam-induced quantum interference effects in a multi-level quantum emitter

H. B. Crispin·N. Talebi
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Abstract

Cathodoluminescence spectroscopy has recently emerged as a novel platform for nanoscale control of nonclassical features of light. Here, we propose a theoretical model for cathodoluminescence from a multi-level quantum emitter. Employing a master equation approach and treating the electron-beam excitation as an incoherent broadband field source, we show that quantum interference can arise between the different relaxation pathways. The induced-interference can significantly modify the time-dependent spectra resulting in the enhancement or suppression of cathodoluminescence. We find that the excitation rate, initial state of the emitter, and excited level spacing play a crucial role in determining the influence of interference. Our findings shed light on electron-beam-induced quantum interference in cathodoluminescence and provides a theoretical basis for exploring quantum optical phenomena in electron-driven multi-level systems.

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H. B. Crispin, N. Talebi. 2025-01-31. Electron-beam-induced quantum interference effects in a multi-level quantum emitter. https://arxiv.org/abs/2501.19230

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