Formation of Frustrated Charge Density Waves in Kagome Metal LuNb$_6$Sn$_6$

F. Z. Yang; X. Huang; Hengxin Tan; A. Kundu; S. Kim; M. Thinel; J. Ingham; A. Rajapitamahuni; C. Nelson; Y. Q. Cai; E. Vescovo; W. R. Meier; D. Mandrus; Brenden R. Ortiz; A. N. Pasupathy; Binghai Yan; H. Miao

arXiv · 2502.20593

Formation of Frustrated Charge Density Waves in Kagome Metal LuNb$_6$Sn$_6$

F. Z. Yang·X. Huang·Hengxin Tan·A. Kundu·S. Kim·M. Thinel·J. Ingham·A. Rajapitamahuni·C. Nelson·Y. Q. Cai·E. Vescovo·W. R. Meier·D. Mandrus·Brenden R. Ortiz·A. N. Pasupathy·Binghai Yan·H. Miao

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Abstract

The charge density wave (CDW), a translational symmetry breaking electronic liquid, plays a pivotal role in correlated quantum materials, such as high-T$_c$ superconductors and topological semimetals. Recently, CDWs that possibly intertwine with superconductivity and magnetism are observed in various kagome metals. However, the nature of CDWs and the role of the Fermi surface (FS) topology in these materials remain an unresolved challenge. In this letter, we reveal the formation of CDWs in the newly discovered kagome metal LuNb$_6$Sn$_6$. We observe a precursor CDW correlation that features a "yield sign"-like hollow triangle diffuse scattering pattern and nearly complete softening of a flat optical phonon band near Q$_H$=(1/3, 1/3, 1/2). The scattering intensity of the precursor CDW displays divergent behavior as decreasing temperature until T$_{CDW}$=70 K, where a competing CDW at Q$_{CDW}$=(1/3, 1/3, 1/3) emerges. Using scanning tunneling microscopy/spectroscopy, we image the frustrated CDW patterns that show a short phase coherence length about ~20 nm in real space. Combined with first principles calculations, our observations support frustrated lattice interactions that are modulated by the FS topology. These results shed light on the interplay between FS and CDW in quantum materials with nearly degenerate structural deformation patterns.

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F. Z. Yang, X. Huang, Hengxin Tan, A. Kundu, S. Kim, M. Thinel, J. Ingham, A. Rajapitamahuni, C. Nelson, Y. Q. Cai, E. Vescovo, W. R. Meier, D. Mandrus, Brenden R. Ortiz, A. N. Pasupathy, Binghai Yan, H. Miao. 2025-02-27. Formation of Frustrated Charge Density Waves in Kagome Metal LuNb$_6$Sn$_6$. https://arxiv.org/abs/2502.20593

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