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arXiv · 2503.07174

Quantum spin dynamics of the honeycomb magnet K$_2$Co$_2$TeO$_6$ in high magnetic fields

Patrick Pilch·Laur Peedu·Urmas Nagel·Toomas Rõõm·Changqing Zhu·Yurii Skourski·Xianghan Xu·Robert J. Cava·Zhe Wang
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Abstract

We present terahertz spectroscopic measurements of quantum spin dynamics in the honeycomb magnet K$_2$Co$_2$TeO$_6$ as a function of temperature, polarization and in an external magnetic field applied in the honeycomb plane. Magnetic excitations are resolved below the magnetic ordering temperature of $T_\text{N}$ = 12 K. In the applied magnetic field, we reveal characteristic field dependence not only for the magnetic excitations observed at zero field, but also a rich set of modes emerging in finite fields. The observed magnetic excitations exhibit clear dependence on the terahertz polarization, and characteristic features at field-induced phase transitions consistent with our high-field magnetization data. We cannot evidently resolve a continuumlike feature, even when the long-range magnetic order is presumably suppressed in the strong magnetic field, indicating that a Kitaev-type interaction, if existing, is subleading in this compound.

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Patrick Pilch, Laur Peedu, Urmas Nagel, Toomas Rõõm, Changqing Zhu, Yurii Skourski, Xianghan Xu, Robert J. Cava, Zhe Wang. 2025-03-10. Quantum spin dynamics of the honeycomb magnet K$_2$Co$_2$TeO$_6$ in high magnetic fields. https://doi.org/10.1103/dnpq-lnrm

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