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arXiv · 2503.10290

Observation of a gapped phase in the one-dimensional $S = {\frac{1}{2}}$ Heisenberg antiferromagnetic chain Cu(Ampy)ClBr

Saikat Nandi·Monika Jawale·Sanjay Bachhar·Rahul Kumar·Marlis Schuller·Rabindranath Bag·J. Wilkinson·Jörg Sichelschmidt·A. Sundaresan·Sara Haravifard·N. Büttgen·A. V. Mahajan
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Abstract

Spin-1/2 Heisenberg antiferromagnetic frustrated spin chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is tuned. We present a comprehensive investigation of the structural, magnetic, and thermodynamics properties of the spin-1/2 compound, Cu(Ampy)ClBr (Ampy= C$_6$H$_8$N$_2$ = 2-(Aminomethyl)pyridine) via x-ray diffraction, magnetization, specific heat, $^1$H nuclear magnetic resonance (NMR), electron spin resonance (ESR), and muon spin relaxation ($\mu$SR) techniques. The crystal structure features an anisotropic triangular chain lattice of magnetic Cu$^{2+}$ ions. Our bulk and local probe experiments detect neither long-range magnetic ordering nor spin freezing down to 0.06 K despite the presence of moderate antiferromagnetic interaction between Cu$^{2+}$ spins as reflected by a Curie-Weiss temperature of about $-9$ K from the bulk susceptibility data. A broad maximum is observed at about 9 K in magnetic susceptibility and specific heat data, indicating the onset of short-range spin correlations. At low temperatures, the zero-field magnetic specific heat and the $^1$H NMR spin-lattice relaxation rate follow an exponential temperature dependence, indicating the presence of gapped magnetic excitations. Furthermore, persistent spin dynamics down to 0.088 K observed by zero-field $\mu$SR evidences lack of any static magnetism.

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Saikat Nandi, Monika Jawale, Sanjay Bachhar, Rahul Kumar, Marlis Schuller, Rabindranath Bag, J. Wilkinson, Jörg Sichelschmidt, A. Sundaresan, Sara Haravifard, N. Büttgen, A. V. Mahajan. 2025-03-13. Observation of a gapped phase in the one-dimensional $S = {\frac{1}{2}}$ Heisenberg antiferromagnetic chain Cu(Ampy)ClBr. https://doi.org/10.1103/mkdv-8m61

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