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arXiv · 2503.21946

Magnetic polarons due to spin-length fluctuations in $\boldsymbol{d}^\mathbf{4}$ spin-orbit Mott systems

Jan Revenda·Krzysztof Wohlfeld·Jiří Chaloupka
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Abstract

Mott insulators based on $4d$ and $5d$ transition-metal ions, where spin-orbit interaction plays a key role, can exhibit various forms of unusual magnetism. A particular example is the antiferromagnet Ca$_2$RuO$_4$ containing $d^4$ Ru$^{4+}$ ions. Here the spin-orbit interaction stabilizes the non-magnetic $J=0$ singlet ionic ground state, which gets dynamically mixed - via exchange interactions - with low-energy $J=1$ ionic excitations. Thanks to a sufficient strength of the exchange, these excitations condense and a long-range order emerges. The resulting ordered moments are soft and prone to fluctuations of their effective length. The corresponding amplitude mode appears as a prominent magnetic excitation and complements the conventional magnons involving rotations of the moments. Motivated by this peculiar kind of magnetic order and the specific spectrum of magnetic excitations, we study their influence on the propagation of doped carriers. To this end, we construct a microscopic model including both $d^4$ and $d^5$ degrees of freedom and address the propagation of an injected electron by employing self-consistent Born approximation. We find that the electron shows a combination of both free and a polaronic type of motion, where the mobile carrier strongly interacts with an accompanying cloud of magnetic excitations. Remarkably, in the latter case it is the exotic excitation - the amplitude mode - that is found to dominate over the contribution of magnons. Our soft-spin situation thus largely contrasts with spin polarons widely discussed in the context of doped Heisenberg-like magnets based on rigid spin moments.

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Jan Revenda, Krzysztof Wohlfeld, Jiří Chaloupka. 2025-03-27. Magnetic polarons due to spin-length fluctuations in $\boldsymbol{d}^\mathbf{4}$ spin-orbit Mott systems. https://doi.org/10.1103/physrevb.111.195125

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