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arXiv · 2503.23704

Paramagnetic half-moon shaped diffuse scattering arising from 3D magnetic frustration

Nelly Natsch·Tara N. Tošić·Jian-Rui Soh·Nicola A. Spaldin
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Abstract

We use spin dynamics simulations to determine the origin of the unusual correlated diffuse scattering, characterised by half-moon shapes bridging the magnetic Bragg peaks, observed in the polarised elastic neutron scattering from manganese tungstate, MnWO\textsubscript{4}. We first fit a Heisenberg Hamiltonian with twelve nearest-neighbour exchange interactions and single-ion anisotropy to the experimental ground-state magnon dispersion. We then show via spin dynamics simulations that our model Hamiltonian both reproduces the experimentally observed half-moon features and captures their persistence into the paramagnetic regime. Moreover, we identify the three-dimensional, competing antiferromagnetic interactions driving this behavior. Our work complements earlier studies of half-moon-shaped signatures in pyrochlore and triangular structures, by providing insight into their origin in a zigzag chain geometry with three-dimensional competing exchange interactions.

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Nelly Natsch, Tara N. Tošić, Jian-Rui Soh, Nicola A. Spaldin. 2025-03-31. Paramagnetic half-moon shaped diffuse scattering arising from 3D magnetic frustration. https://arxiv.org/abs/2503.23704

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