Light-Induced Spin Slanting in 2D Multiferroic Magnet

Jiangyu Zhao; Yangyang Feng; Kaiying Dou; Xinru Li; Ying Dai; Baibiao Huang; Yandong Ma

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arXiv · 2504.08185

Light-Induced Spin Slanting in 2D Multiferroic Magnet

Jiangyu Zhao·Yangyang Feng·Kaiying Dou·Xinru Li·Ying Dai·Baibiao Huang·Yandong Ma

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Abstract

Controlling spin orientation of two-dimensional (2D) materials has emerged as a frontier of condensed-matter physics, resulting in the discovery of various phases of matter. However, in most cases, spin orientation can be stablished only at specific directions of out-of-plane and in-plane, which is a drawback compared with three-dimensional systems, limiting exploration of novel physics. Here, we introduce a methodology for manipulating spin slanting in 2D multiferroic materials through ultrafast pulses of light. Based on model analysis, we find that simultaneous triggering spin-orbit coupling induced interactions from in-plane and out-of-plane orbitals can generate spin slanting. By choosing 2D multiferroic materials with specific low-energy composition endowed by symmetry, such triggering can be readily achieved through ultrafast light illumination, leading to light-induced spin slanting. Using real-time time-dependent density-functional theory, we demonstrate this approach in multiferroic single-layer CuCr2Se4. This study provides an efficient way to manipulate spin orientation in 2D materials and establishes a general platform to explore physics and applications associated with spin slanting.

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Jiangyu Zhao, Yangyang Feng, Kaiying Dou, Xinru Li, Ying Dai, Baibiao Huang, Yandong Ma. 2025-04-11. Light-Induced Spin Slanting in 2D Multiferroic Magnet. https://arxiv.org/abs/2504.08185

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