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arXiv · 2505.04824

Theoretical perspectives on optical control of magnetism in spin-charge coupled systems

Masahito Mochizuki
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Abstract

In this article, we review recent theoretical research on photocontrol of magnetism in several spin-charge coupled systems. The control of magnetism with light has been a central issue in condensed-matter physics, attracting enormous research interest both for fundamental science and for technological applications. This field of research has developed rapidly in recent years along with the development of laser technology. However, because the direct coupling between the light magnetic field and magnetization via the Zeeman coupling is very weak in terms of the energy scale, it is, in principle, difficult to induce dramatic effects as far as this magnetic light-matter interaction is exploited. On the contrary, the interaction between the light electric field and electron charges has an energy scale two to three orders of magnitude larger than that of the magnetic interaction. Therefore, we may realize astonishing photoinduced physical phenomena and novel optical device functions by exploiting this electric light-matter interaction. Spin-charge coupled magnets, e.g., double-exchange magnets, multiferroics materials, and Rashba electron systems, in which spins and charges are strongly coupled through several kinds of mechanisms such as exchange interactions and spin-orbit coupling, are ideal systems for realizing this idea. Recent theoretical studies have revealed that it is possible to control, manipulate and switch the magnetization coupled to electron charges in these systems through exciting and/or driving them with light electric fields. The following three recent topics are discussed as examples of such theoretical studies, that is, photoinduced magnetic phase transitions in irradiated double-exchange models, highly efficient photoinduction of spin polarization in Rashba electron systems, and electromagnon excitations and their intense excitation effects in multiferroic materials.

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Masahito Mochizuki. 2025-05-07. Theoretical perspectives on optical control of magnetism in spin-charge coupled systems. https://arxiv.org/abs/2505.04824

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