Orbital-Selective Band Structure Evolution in BaFe$_{2-x}$M$_x$As$_2$ (M = Cr, Co, Cu, Ru and Mn) Probed by Polarization-Dependent ARPES

Abstract

We present a systematic study of the evolution of the band structure in the Fe-based superconductor family BaFe$_{2-x}$M$_x$As$_2$ (M = Cr, Co, Cu, Ru and Mn) using polarization-dependent angle-resolved photoemission spectroscopy (ARPES). Low-substituted samples, with comparable spin-density wave transition temperatures ($T_\text{SDW}$), were chosen to facilitate controlled comparisons. The sizes of the central hole pockets ($\alpha$, $\beta$, and $\gamma$) remain largely unchanged across different substitutions, showing no clear correlation with either $T_\text{SDW}$ or the As height relative to the Fe planes. However, subtle trends are observed: a modest increase in the size of the $\eta_\text{X}$ electron pocket correlates with the suppression of $T_\text{SDW}$. Furthermore, the contraction of the $\eta_\text{X}$ pocket appears to be linked to an increase in the As height relative to the Fe planes. Our results suggest that the suppression of $T_\text{SDW}$ is primarily driven by changes in the Fe-As bond length, with the effect being more pronounced in electronic states with planar character. These findings provide insight into the electronic structure of BaFe$_{2-x}$M$_x$As$_2$.