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arXiv · 2510.00970

Cumulant expansion approach to the decay dynamics of interacting M\"ossbauer nuclei after strong impulsive excitation

Miriam Gerharz·Jörg Evers
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Abstract

Recent progress in accelerator-based x-ray sources brings higher excitation of ensembles of M\"ossbauer nuclei closer to experimental feasibility. Yet, a theoretical modeling of the decay dynamics of the interacting nuclear ensemble after the impulsive excitation is still an open challenge. Here, we derive a set of nonlinear equations which is capable of efficiently modeling large nuclear ensembles for arbitrary degrees of excitation. As key signature for higher excitation, we identify a non-linear time-evolution of the nuclear dipole phase, which can be tuned via the scattering geometry, and interferometrically be measured. Furthermore, we identify interesting finite-size effects in the nuclear dynamics of small ensembles. Our results provide important guidance for future experiments aiming at the non-linear excitation of nuclei. We further envision the exploration of finite size-effects in M\"ossbauer spectroscopy with highest spatial resolution, i.e., small sample volumes.

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Miriam Gerharz, Jörg Evers. 2025-10-01. Cumulant expansion approach to the decay dynamics of interacting M\"ossbauer nuclei after strong impulsive excitation. https://arxiv.org/abs/2510.00970

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