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arXiv · 2511.10246

Direct Raman observation of the quantum metric in a quantum magnet

Chao-Fan Wang·Han Ge·Jun-Yang Chen·Liusuo Wu·Xiaobin Chen·Jia-Wei Mei·Mingyuan Huang
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Abstract

The quantum geometric tensor (QGT) unifies the Berry curvature (its imaginary part) and the quantum metric (its real part), yet Raman studies of chiral phonons have so far accessed only the former. We perform circularly polarized Raman spectroscopy on the quantum magnet K2Co(SeO3)2, where the field-odd chiral splitting and the field-even center-frequency shift collapse onto a single curve across temperature and magnetic field, revealing a common microscopic origin for both observables. Since the chiral splitting reflects the Berry curvature, the concomitant even component, arising from the same microscopic origin, captures the field-induced change of the quantum metric, corresponding to the diagonal Born-Oppenheimer correction. Across two resolvable Eg modes, the unified data are well captured by a simple empirical quadratic relation. These results establish Raman spectroscopy as a direct probe of the quantum metric and an operational decomposition of quantum geometry within a single measurement.

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Chao-Fan Wang, Han Ge, Jun-Yang Chen, Liusuo Wu, Xiaobin Chen, Jia-Wei Mei, Mingyuan Huang. 2025-11-13. Direct Raman observation of the quantum metric in a quantum magnet. https://arxiv.org/abs/2511.10246

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