SearcharxivSearch

arXiv · 2511.16220

Diffuse Laser Cooling Based on the $6\mathrm{P}_{3/2}$ Excited State of Rubidium Atoms via 420 nm Blue Light

Abstract

To date, the laser cooling of rubidium atoms has inevitably relied on 780 nm cooling light corresponding to the first excited state $5\mathrm{P}_{3/2}$. Surprisingly, we demonstrate laser cooling directly utilizing 420 nm blue light for active optical clock, which corresponds to the high excited state $6\mathrm{P}_{3/2}$ of Rb atom. Experimentally, we successfully apply the 420 nm diffuse laser cooling technique to prepare a cold $^{87}\mathrm{Rb}$ atomic cloud with a length of up to one meter, and measure the cold-atom absorption spectroscopy. The cold atom number is approximately $4.4\times10^{7}$. We systematically compare the cooling effects of 420 nm and 780 nm diffuse laser cooling, and verify the feasibility of blue light cooling using high excited state. This work directly employs blue light to cool and manipulate ground-state Rb atoms to the 6P excited state, providing a new and efficient approach for the cold-atom active optical clock. It is also expected to open up research directions and application prospects in frontier fields such as Rydberg atoms, ultracold quantum gases Bose-Einstein condensation, quantum information, and so on.

Explore related subjects

Keep this discovery

BibTeXRIS

Jia Zhang, Xun Gao Zheng Xiao, Xiaolei Guan Ruihang Chen, Mengyuan Han Tiantian Shi, Jingbiao Chen. 2025-11-20. Diffuse Laser Cooling Based on the $6\mathrm{P}_{3/2}$ Excited State of Rubidium Atoms via 420 nm Blue Light. https://arxiv.org/abs/2511.16220

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Delay-engineered dynamical phases in a programmable non-Markovian spin oscillator

Non-Markovian dynamics offer a new route towards engineering non-equilibrium matter, where memory and feedback act as programmable resources for controlling order in time. Here we report the realization of a non-Markovian spin oscillator in a hot vapour $^{129}$Xe-Cs co-magnetometer with programmable feedback delay and gain. By tuning these parameters, we observe a hierarchy of dynamical phases, including time-crystalline response, nonlinear bifurcations, and frequency-comb formation. The measured spectra and phase boundaries are captured by linear stability analysis of delayed Bloch equations, revealing these phenomena as different manifestations of the same memory-induced instability structure. These results establish time-delayed feedback as a powerful strategy for controlling non-equilibrium phases, enabling quantum sensing, frequency referencing, and synchronization within a single spin-based platform.

physics.atom-ph

Non-stick vacuum wall collisions with a laser-coolable molecule

Molecular species that are suitable for direct laser cooling are typically considered lost or destroyed if they collide with an ambient temperature vacuum wall. Here, we study surface collisions with aluminum monofluoride (AlF), a laser-coolable molecule that survives this process with unusually high probability. We detect the outgoing AlF molecules from a single wall collision via Doppler-sensitive laser-induced fluorescence spectroscopy, using incoming supersonic (pulsed) and thermochemical (continuous) molecular beams. The angular, velocity and rovibrational level distributions of the outgoing molecules show near-complete thermalisation to the wall in a single collision event. We determine an upper limit to the surface residence time of about 5$~\mu$s, and by monitoring the decay in density of pulses of molecules loaded into a small storage volume, we deduce the surface sticking probability for different materials. For a siloxane-coated metallic surface, the sticking probability of AlF is about 0.015, allowing us to accumulate molecules from the thermochemical source into an ambient temperature storage vessel at densities near $10^{8}~$cm$^{-3}$. This provides a route to compact, portable traps for neutral molecules.

physics.atom-ph

Kinetic modeling of molecular beam formation in a cryogenic buffer-gas cell

Cryogenic buffer-gas cells are widely used to produce cold molecular beams, but the microscopic dynamics governing beam formation remain challenging to model. Here we present fully kinetic simulations of a cryogenic buffer-gas cell using the Direct Simulation Monte Carlo method implemented in the PICLas framework, treating the buffer gas and ablated molecules within a single unified model. We capture characteristic features of cryogenic buffer-gas sources, including plume cooling, directed transport toward the aperture, and the formation of a slow molecular beam, while also resolving energy transfer from the hot ablation plume to the helium buffer gas that is inaccessible to existing approaches relying on the background-gas approximation. Our results demonstrate that fully kinetic simulations can provide detailed insights into buffer-gas cell dynamics and open a route toward a systematic optimization of such sources.

physics.atom-ph