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arXiv · 2512.24781

Non-equilibrium pathways between cluster morphologies in active phase separation: necking, rupture and cavitation

Liheng Yao·Michael E. Cates·Robert L. Jack
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Abstract

We investigate the dynamical pathways of a morphological transition in a two-dimensional active lattice gas undergoing motility-induced phase separation. The transition is between two locally stable morphologies of the liquid cluster: a system-spanning "slab" and a compact "droplet". We generate trajectories of this transition in both directions using forward flux sampling. We find that the droplet-to-slab transition always follows a similar mechanism to its equilibrium counterpart, but the reverse (slab-to-droplet) transition depends on rare non-equilibrium fluctuations. At low P\'eclet numbers the equilibrium and non-equilibrium pathways compete, while at high P\'eclet numbers the equilibrium pathway is entirely suppressed, and the only allowed mechanism involves a large vapour bubble. We discuss the implications of these findings for active matter systems more generally.

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Liheng Yao, Michael E. Cates, Robert L. Jack. 2025-12-31. Non-equilibrium pathways between cluster morphologies in active phase separation: necking, rupture and cavitation. https://doi.org/10.1103/vdps-lhr9

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