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arXiv · 2603.20709

Crystal Growth and anisotropic magneto-transport properties of semimetallic LaNiSb3

Haribrahma Singh·Aarti Gautam·Prabuddha Kant Mishra·Rie Y. Umetsu·Ashok Kumar Ganguli
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Abstract

Single crystals of LaNiSb$_3$ were grown using the Sn flux method. Structural characterization confirms that LaNiSb$_3$ crystallizes in the orthorhombic $Pbcm$ space group with lattice parameters $a = 13.0970(2)\,\mathrm{\AA}$, $b = 6.1400(4)\,\mathrm{\AA}$, and $c = 12.1270(4)\,\mathrm{\AA}$. Electrical resistivity measurements demonstrate metallic behavior over the entire temperature range of 3--300~K. The magnetoresistance exhibits a positive anisotropic response, attaining a maximum of $\sim 8\%$ for $H \parallel b$, with a pronounced crossover from quadratic to nearly linear field dependence. Angular-dependent MR measurements reveal a pronounced twofold symmetry upon magnetic field rotation within both the $ab$ and $ac$ crystallographic planes up to 50~K, indicating anisotropic charge transport. Hall resistivity measurements show predominantly electron-type conduction at high temperatures, with an increasing hole contribution upon cooling. The multiband character is further corroborated by the violation of Kohler's scaling and is well described within a semiclassical two-band framework. Collectively, these results suggest that LaNiSb$_3$ exhibits anisotropic multiband electronic transport and is a compelling candidate for exploring structure--property correlations in topological semimetals.

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Haribrahma Singh, Aarti Gautam, Prabuddha Kant Mishra, Rie Y. Umetsu, Ashok Kumar Ganguli. 2026-03-21. Crystal Growth and anisotropic magneto-transport properties of semimetallic LaNiSb3. https://doi.org/10.1063/5.0331991

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