Magneto-ionic control of topological transport in SrRuO3 via band topology engineering

Abstract

The interplay between spin-orbit coupling (SOC) and nontrivial band topology in ferromagnets gives rise to a rich landscape of topological transport phenomena such as anomalous Hall effect (AHE) and topological Hall effect (THE). One central goal in modern spintronics lies in the realization of the active control over topological transport phenomena in a reversible fashion, while unambiguously disentangling respective contributions of THE and AHE to the net Hall effect remains a formidable challenge. Here we establish magneto ionic control as a powerful paradigm for dynamically engineering topological transports in a 4d-orbital SrRuO3 system with sizable SOC and itinerant ferromagnetism. Harnessing controllable protonation or oxygen vacancy incorporation, the Fermi-level upshift relative to avoided band crossings are realized through band filling control, giving rise to tunable reversal temperature of AHE polarity. Of particular note is the emergence of hump like Hall anomalies through extensive ionic doping that can be reversibly switched, irrespective of AHE polarity, providing evidence for a THE signal driven by broken inversion symmetry rather than a two channel AHE. Our findings provide a viable tuning knob for Berry curvature engineering, enabling on demand control of topological transports in strong SOC ferromagnets for low power, reconfigurable all oxide spintronic devices.