Mid- and long-wavelength infrared computational ghost spectroscopy

Abstract

Spectral-domain ghost imaging enables high-resolution spectroscopy with a single-pixel detector. The technique does not rely on spectrally resolved detectors, which makes it inherently robust against turbulence and particularly adapted to weak-light conditions. These features are very attractive for spectral imaging in the mid-infrared region which hosts numerous molecular absorption features but lacks highly sensitive detectors. The implementation of spectral ghost imaging in the mid-infrared has however been limited by the absence of suitable light sources and detectors capable of generating and measuring spectral fluctuations in real time. Here, we demonstrate spectral-domain computational ghost imaging in the mid-infrared based on a nonlinear frequency downconversion scheme. Pre-programmed spectral patterns imposed on broadband light at 1.5 mm using a programmable spectral filter are transferred into the mid-infrared through difference-frequency generation in a nonlinear crystal. This enables computational ghost spectroscopy with a spectral resolution of 0.62 cm-1 using a single-pixel mid-infrared detector. The method is flexible, broadly applicable and, as proof of concept, we demonstrate ghost spectroscopy in mid-wavelength infrared and long-wavelength infrared bands using the nonlinear frequency conversion in chirped-poling lithium niobate and ZnGeP2 crystals, respectively. Our approach provides a new avenue for mid-infrared spectroscopy, remote sensing and spectral imaging.