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arXiv · 2607.19868

Band Engineering of Exciton Polaritons in Resonant Polaritonic Metasurfaces

Polina Pantiukhina·Daria Smirnova·Kirill Koshelev
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Abstract

Polaritonic metasurfaces provide a versatile platform for engineering hybrid light-matter states through the interplay of optical resonances and excitonic excitations. Yet, predictive models often remain phenomenological and rely on coupled-mode equations. Here, we develop an effective Hamiltonian framework for exciton polaritons in resonant polaritonic metasurfaces, derived from a semiclassical single-pole description of excitonic polarization and a Green's-function description of guided-mode resonances. The resulting non-Hermitian Hamiltonian rigorously incorporates resonant photonic harmonics, multiple excitonic degrees of freedom, and radiative losses. The model reveals selection rules governing photonic-excitonic coupling classified by orbital multipole index and polarization, and shows that the minimal number of excitonic degrees of freedom equals the number of relevant photonic modes. We apply the framework to a bulk van der Waals WS$_2$ metasurface patterned into a hexagonal lattice of triangular holes and uncover a new geometry-controlled topological transition driven by dipole-quadrupole band inversion, distinct from the conventional breathing-honeycomb-lattice transition. Full-wave simulations confirm the predicted topological phase diagram and the emergence of photonic and polaritonic edge states at a topological interface. Our results establish a theoretical multimode framework for geometry-controlled bandstructure engineering in polaritonic metasurfaces, with applications in topological, chiral, and quantum integrated photonics.

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Polina Pantiukhina, Daria Smirnova, Kirill Koshelev. 2026-07-22. Band Engineering of Exciton Polaritons in Resonant Polaritonic Metasurfaces. https://arxiv.org/abs/2607.19868

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