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arXiv · 2607.25263

Low-Temperature Magnetoresistance Hysteresis in Granular Cr1-xFexO2: Slow Relaxation of Transport-Active Magnetic Configurations

Abstract

Low-temperature magnetoresistance loops of compacted CrO2 powders become strongly nonmonotonic when electrical transport is dominated by a small number of spin-dependent intergranular tunnelling paths. We reanalyse previously reported data for undoped CrO2 and Fe-containing Cr1-xFexO2, focusing on additional branch crossings beyond the conventional low-field hysteresis. In the Fe-containing specimen, the resistance decreases, passes through a minimum, rises over an extended field interval, and then decreases again at higher field. This nonmonotonic hysteretic feature is strongly reduced when the magnetic-field sweep is slowed. Digitization of the three fastest sweeps shows that the field at which the resistance starts to recover shifts approximately linearly with sweep rate, corresponding to an effective magnetotransport relaxation time of about 3 s. This scale is attributed not to microscopic spin flips but to the slow evolution of local moment and domain configurations at the intergranular contacts dominating the current. The observations are consistent with conventional negative tunnelling magnetoresistance superimposed on a slower resistance-increasing contribution associated with transient local magnetic disorder. Fe increases coercivity and interfacial magnetic heterogeneity while reducing the overall negative magnetoresistance. The results support a transport-weighted magnetic-reconfiguration mechanism for the unusual hysteresis shape.

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BibTeXRIS

E. Yu. Beliayev, V. A. Horielyi, I. G. Mirzoiev, V. V. Andrievskii. 2026-07-28. Low-Temperature Magnetoresistance Hysteresis in Granular Cr1-xFexO2: Slow Relaxation of Transport-Active Magnetic Configurations. https://arxiv.org/abs/2607.25263

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