Searcharxiv⌕ Search

arXiv · 2609.30871

Systematic Evolution of Magnetic Anisotropy and Crystal-electric-field Ground States in SmTr2Ge2

Abstract

We investigated the crystal-electric-field (CEF) states in SmTr2Ge2 (Tr= Co-Cu and Ag) with the ThCr2Si2-type structure by magnetization and specific heat measurements. The magnetic anisotropy evolves systematically with Tr, changing from an easy ab plane for Tr = Co and Ni to an easy c axis for Tr = Cu and Ag. Combined analyses of the low-temperature susceptibility and magnetic entropy indicate a level crossing of the CEF ground state between Ni and Cu, together with a systematic evolution of the first excited CEF energy. The evolution of the magnetic properties correlates with changes in local structural parameters, providing an experimental basis for discussing how the ligand environment around the Sm ion is related to the 4f electronic state.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Ryuji Higashinaka, Kokoro Higo, Tatsuma D. Matsuda, Yuji Aoki. 2026-09-25. Systematic Evolution of Magnetic Anisotropy and Crystal-electric-field Ground States in SmTr2Ge2. https://doi.org/10.7566/jpsj.95.104711

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Charge order before superconductivity in the doped kagome Dirac spin liquid

Doping a quantum spin liquid is expected to produce a superconductor. We show that for the Dirac spin liquid on the kagome lattice the doped charge orders first. The charge is carried by a chargon doublet whose two gauge components are degenerate on the square and triangular lattices, and the kagome lattice, as the line graph of the honeycomb lattice, splits them. One component disperses and condenses in four valleys. The other has flat lowest bands and stays empty over a window in the bare mass whose width, $(\sqrt6-1)t$, follows from the band structure alone. Within that window, in the mean-field chargon theory constructed from the projective symmetry group of the spin liquid, the doped state forms charge and loop-current crystals with the electromagnetic U(1) unbroken and no superconductivity. Pairing requires a gapped descendant of the spin liquid as the parent and then takes the form of a pair-density wave, with no uniform $d+id$ channel at leading order and none at any order for the crystals at the $M$ point. The predicted charge order is odd under the twofold rotation and has no cubic invariant, which distinguishes it from the charge order of the kagome metals.

cond-mat.str-el↗

Multiorbital periodic Anderson model for CeRh2As2

CeRh2As2 is a heavy-fermion superconductor that exhibits distinct low- and high-field superconducting phases, widely interpreted as reflecting a field-induced change in the parity of the order parameter. However, the superconductivity develops in close proximity to magnetic order whose microscopic origin and nature remain unclear. Moreover, the low-lying crystal-electric-field-split doublets of the Ce 4f electrons appear to realize an unusual "quasi-quartet" structure. This has motivated proposals that quadrupolar degrees of freedom play an important role in the low-temperature physics. Here we develop a microscopic heavy-fermion description of CeRh2As2 that incorporates both the quasi-quartet structure and the nonsymmorphic symmetry. Within a multiorbital periodic Anderson model, we include the lowest-lying $Γ_7$ and $Γ_6$ doublets of the Ce 4f electrons, and allow for nonlocal hybridization with the conduction d electrons. Single occupancy of the 4f states is enforced within the rotationally invariant slave-boson formalism. Adopting a mean-field treatment, we first show that the effective low-energy Hamiltonian is accurately captured by a single-orbital tight-binding model, justifying the minimal descriptions widely employed in the literature. Allowing for a magnetic ground state, we find that our model displays metallic $\mathbf{Q}=(π,π)$ antiferromagnetic order over a wide parameter regime. Ferromagnetic solutions also occur, but in a smaller region of parameter space and with greater sensitivity to carrier concentration and the form of the f-d hybridization. Quadrupolar moments appear only within magnetically ordered phases and are generally small, becoming substantial only when the $Γ_7$ and $Γ_6$ doublets are nearly degenerate. Our results provide a microscopic basis for understanding the itinerant heavy-fermion physics and ordered phases of CeRh2As2.

cond-mat.str-el↗

Altermagnetic phases and phase transitions in Lieb-$5$ Hubbard model

The emergence of altermagnetism, the collinear magnetic phase characterized by momentum-dependent spin-split bands but zero net magnetization, has fundamentally reshaped the classification of magnetic order. We propose an altermagnetic (AM) order in a repulsive Hubbard model on the Lieb-$5$ lattice. Considering only nearest-neighbor hoppings within the lattice, we show a phase transition from the nonmagnetic to a unique AM isolated band metal phase (AMIM), allowing clear identification of spin-split states. Additionally, the AM metallic phase (AMM) is also shown to appear as an intermediate phase during the transition from the normal metal to the AMIM in the presence of the diagonal hopping within each unit cell of the Lieb-$5$ lattice. The manifestation of distinct AM phases and the phase transitions, driven by Hubbard interaction and hopping integrals, have been explored in terms of spin-resolved band structure, spectral function, and the behavior of the AM order parameter. The stability of these AM phases against the spin-orbit coupling and temperature is also established.

cond-mat.str-el↗