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Resonance Raman scattering in semiconductor quantum dots: Adiabatic vs. time-dependent perturbation theory

E. Menendez-Proupin·Nana Cabo-Bisset
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Abstract

The adiabatic theory of resonance one-phonon Raman scattering in semiconductor nanocrystals is revised and extended with perturbative non-adiabatic corrections, given by the Albrecht's B term. This theory is confronted with the time-dependent perturbation approach, pointing at their differences and similarities. It is shown that both theories are equivalent in the limit of weak electron-phonon coupling and non-degenerate or uncoupled resonant states. Evaluations of the A and B terms for the confined LO phonon in CdSe and CdS nanocrystals are reported. These evaluations show that the B term can usually be neglected.

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E. Menendez-Proupin, Nana Cabo-Bisset. 2002-04-26. Resonance Raman scattering in semiconductor quantum dots: Adiabatic vs. time-dependent perturbation theory. https://doi.org/10.1103/physrevb.66.085317

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