Delocalization of Wannier-Stark ladders by phonons: tunneling and stretched polarons

Abstract

We study the coherent dynamics of a Holstein polaron in strong electric fields. A detailed analytical and numerical analysis shows that even for small hopping constant and weak electron-phonon interaction, polaron states can become delocalized if a resonance condition develops between the original Wannier-Stark states and the phonon modes, yielding both tunneling and `stretched' polarons. The unusual stretched polarons are characterized by a phonon cloud that {\em trails} the electron, instead of accompanying it. In general, our novel approach allows us to show that the polaron spectrum has a complex nearly-fractal structure, due to the coherent coupling between states in the Cayley tree which describes the relevant Hilbert space. The eigenstates of a finite ladder are analyzed in terms of the observable tunneling and optical properties of the system.