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Long range magnetic ordering in a spin-chain compound, Ca$_3$CuMnO$_6$, with multiple bond distances

Kausik Sengupta·S. Rayaprol·K. K. Iyer·E. V. Sampathkumaran
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Abstract

The results of ac and dc magnetization and heat capacity measurements as a function of temperature (T = 1.8 to 300 K) are reported for a quasi-one-dimensional compound, Ca$_3$CuMnO$_6$, crystallizing in a triclinically distorted K$_4$CdCl$_6$-type structure. The results reveal that this compound undergoes antiferromagnetic ordering close to 5.5 K. In addition, there is another magnetic transition below 3.6 K. Existence of two long-range magnetic transitions is uncommon among quasi-one-dimensional systems. It is interesting to note that both the magnetic transitions are of long-range type, instead of spin-glass type, in spite of the fact that the Cu-O and Mn-O bond distances are multiplied due to this crystallographic distortion. In view of this, this compound could serve as a nice example for studying "order-in-disorder" phenomena.

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Kausik Sengupta, S. Rayaprol, K. K. Iyer, E. V. Sampathkumaran. 2003-06-06. Long range magnetic ordering in a spin-chain compound, Ca$_3$CuMnO$_6$, with multiple bond distances. https://doi.org/10.1103/physrevb.68.012411

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