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A common behavior of thermoelectric layered cobaltites: incommensurate spin density wave states in [Ca$_2$Co$_{4/3}$Cu$_{2/3}$O$_4$]$_{0.62}$[CoO$_2$] and [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$]

J. Sugiyama·J. H. Brewer·E. J. Ansaldo·H. Itahara·K. Dohmae·C. Xia·Y. Seno·B. Hitti·T. Tani
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Abstract

Magnetism of a misfit layered cobaltite [Ca$_2$Co$_{4/3}$Cu$_{2/3}$O$_4$]$_x^{\rm RS}$[CoO$_2$] ($x \sim$ 0.62, RS denotes a rocksalt-type block) was investigated by a positive muon spin rotation and relaxation ($μ^+$SR) experiment. A transition to an incommensurate ({\sf IC}) spin density wave ({\sf SDW}) state was found below 180 K (= $T_{\rm C}^{\rm on}$); and a clear oscillation due to a static internal magnetic field was observed below 140 K (= $T_{\rm C}$). Furthermore, an anisotropic behavior of the zero-field $μ^+$SR experiment indicated that the {\sf IC-SDW} propagates in the $a$-$b$ plane, with oscillating moments directed along the c axis. These results were quite similar to those for the related compound [Ca$_2$CoO$_3$]$_{0.62}^{\rm RS}$[CoO$_2$], {\sl i.e.}, Ca$_3$Co$_4$O$_9$. Since the {\sf IC-SDW} field in [Ca$_2$Co$_{4/3}$Cu$_{2/3}$O$_4$]$_{0.62}^{\rm RS}$[CoO$_2$] was approximately same to those in pure and doped [Ca$_2$CoO$_3$]$_{0.62}^{\rm RS}$[CoO$_2$], it was concluded that the {\sf IC-SDW} exist in the [CoO$_2$] planes.

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J. Sugiyama, J. H. Brewer, E. J. Ansaldo, H. Itahara, K. Dohmae, C. Xia, Y. Seno, B. Hitti, T. Tani. 2003-11-07. A common behavior of thermoelectric layered cobaltites: incommensurate spin density wave states in [Ca$_2$Co$_{4/3}$Cu$_{2/3}$O$_4$]$_{0.62}$[CoO$_2$] and [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$]. https://doi.org/10.1088/0953-8984%2F15%2F49%2F031

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