SearcharxivSearch

arXiv · cond-mat/0406142

Dependence of the superconducting critical temperature on the number of layers in homologous series of high-Tc cuprates

Abstract

We study a model of $n$-layer high-temperature cuprates of homologous series like HgBa_2Ca_(n-1)Cu_nO_(2+2n+δ) to explain the dependence of the critical temperature Tc(n) on the number $n$ of Cu-O planes in the elementary cell. Focusing on the description of the high-temperature superconducting system in terms of the collective phase variables, we have considered a semi-microscopic anisotropic three-dimensional vector XY model of stacked copper-oxide layers with adjustable parameters representing microscopic in-plane and out-of-plane phase stiffnesses. The model captures the layered composition along c-axis of homologous series and goes beyond the phenomenological Lawrence-Doniach model for layered superconductors. Implementing the spherical closure relation for vector variables we have solved the phase XY model exactly with the help of transfer matrix method and calculated Tc(n) for arbitrary block size $n$, elucidating the role of the c-axis anisotropy and its influence on the critical temperature. Furthermore, we accommodate inhomogeneous charge distribution among planes characterized by the charge imbalance coefficient $R$ being the function of number of layers $n$. By making a physically justified assumption regarding the doping dependence of the microscopic phase stiffnesses, we have calculated the values of parameter $R$ as a function of block size $n$ in good agreement with the nuclear magnetic resonance data of carrier distribution in multilayered high-Tc cuprates.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

T. A. Zaleski, T. K. Kopec. 2004-06-05. Dependence of the superconducting critical temperature on the number of layers in homologous series of high-Tc cuprates. https://doi.org/10.1103/physrevb.71.014519

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Out-of-equilibrium relaxation dynamics of the superconducting order parameter in CsV$_3$Sb$_5$

The application of a time-varying strain field drives a superconducting order parameter out of equilibrium. How the order parameter relaxes back to equilibrium depends both on the structure of the superconducting gap and on the nature of quasiparticle scattering. We report the discovery of an ultrasonic attenuation peak inside the superconducting state of the kagome superconductor CsV$_3$Sb$_5$. This peak is the natural consequence of the order parameter relaxation time matching the ultrasonic drive frequency near $T_{\rm c}$. From the measured frequency dependence of the peak, we extract a microscopic scattering time of $\tau_N = 25$ ps. This timescale is two orders of magnitude longer than the elastic scattering time as determined by resistivity measurements, but is comparable to the inelastic scattering time determined by thermal transport. Within the conventional framework of order-parameter relaxation, this implies that elastic scattering is ineffective at relaxing the superconducting condensate, consistent with a sign-preserving $s$-wave state obeying Anderson's theorem.

cond-mat.supr-con

Eight-unit-cell electronic modulations in cuprates originating from local molecular orbitals

The pair density wave (PDW) state with eight-unit-cell (8a0) periodicity has been widely regarded as the primary order in cuprates, yet its existence and origin remain subjects of intense debate. Using spectroscopic imaging scanning tunneling microscopy, we observe spatial modulations of the electronic states with approximately 8a0 periodicity in both the superconducting and insulating regimes of hole-doped Ca2CuO2Cl2 cuprate. We find that the 8a0 spatial patterns are generated by the formation of molecular orbitals by doped holes, which organize into 4a0*4a0 plaquettes as the basic unit. Our results identify the 4a0 molecular orbital as the fundamental electronic building block in cuprates, while the 8a0 PDW represents a spatial subharmonic that emerges at sufficiently high doping.

cond-mat.supr-con

Record-Breaking Elemental Superconductivity in Tetralayer Kagome Borophene

Superconductivity above the liquid-nitrogen temperature remains rare in two-dimensional elemental crystals, where strong covalent bonding often yields high phonon frequencies but insufficient electron-phonon coupling. Here, using first-principles calculations and fully anisotropic Migdal-Eliashberg theory, we predict tetralayer kagome borophene (TKB) stabilized by ABAB covalent stacking, as a liquid-nitrogen-temperature elemental superconductor. With a predicted critical temperature of 102 K, TKB sets a record-high value among previously reported elemental superconductors. Unlike known high-Tc boron-based superconductors dominated by in-plane sigma-bonding states and high-frequency in-plane B-B stretching modes, TKB realizes an out-of-plane s-pz-bonding-mediated pairing mechanism, in which interlayer s-pz bonding states at the Fermi level are strongly coupled to low-frequency out-of-plane vibrations of boron atoms. These results reveal a distinct out-of-plane pairing channel in multilayer borophene and establish covalent stacking engineering as a potential route for high-Tc superconductivity in two-dimensional materials.

cond-mat.supr-con