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Theory for transport through a single magnetic molecule: Endohedral N@C60

Florian Elste·Carsten Timm
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Abstract

We consider transport through a single N@C60 molecule, weakly coupled to metallic leads. Employing a density-matrix formalism we derive rate equations for the occupation probabilities of many-particle states of the molecule. We calculate the current-voltage characteristics and the differential conductance for N@C60 in a break junction. Our results reveal Coulomb-blockade behavior as well as a fine structure of the Coulomb-blockade peaks due to the exchange coupling of the C60 spin to the spin of the encapsulated nitrogen atom.

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Florian Elste, Carsten Timm. 2005-04-19. Theory for transport through a single magnetic molecule: Endohedral N@C60. https://doi.org/10.1103/physrevb.71.155403

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