Searcharxiv⌕ Search
Home/Archive/arXiv

arXiv · cond-mat/0503558

Raman Response of Magnetic Excitations in Cuprate Ladders and Planes

K. P. Schmidt·A. Gössling·U. Kuhlmann·C. Thomsen·A. Löffert·C. Gross·W. Assmus
View original source ↗Read source document ↗Export metadata ↓

Abstract

An unified picture for the Raman response of magnetic excitations in cuprate spin-ladder compounds is obtained by comparing calculated two-triplon Raman line-shapes with those of the prototypical compounds SrCu2O3 (Sr123), Sr14Cu24O41 (Sr14), and La6Ca8Cu24O41 (La6Ca8). The theoretical model for the two-leg ladder contains Heisenberg exchange couplings J_parallel and J_perp plus an additional four-spin interaction J_cyc. Within this model Sr123 and Sr14 can be described by x:=J_parallel/J_perp=1.5, x_cyc:=J_cyc/J_perp=0.2, J_perp^Sr123=1130 cm^-1 and J_perp^Sr14=1080 cm^-1. The couplings found for La6Ca8 are x=1.2, x_cyc=0.2, and J_perp^La6Ca8=1130 cm^-1. The unexpected sharp two-triplon peak in the ladder materials compared to the undoped two-dimensional cuprates can be traced back to the anisotropy of the magnetic exchange in rung and leg direction. With the results obtained for the isotropic ladder we calculate the Raman line-shape of a two-dimensional square lattice using a toy model consisting of a vertical and a horizontal ladder. A direct comparison of these results with Raman experiments for the two-dimensional cuprates R2CuO4 (R=La,Nd), Sr2CuO2Cl2, and YBa2Cu3O(6+delta) yields a good agreement for the dominating two-triplon peak. We conclude that short range quantum fluctuations are dominating the magnetic Raman response in both, ladders and planes. We discuss possible scenarios responsible for the high-energy spectral weight of the Raman line-shape, i.e. phonons, the triple-resonance and multi-particle contributions.

Explore related subjects

cond-mat.str-elcond-mat.supr-con

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

K. P. Schmidt, A. Gössling, U. Kuhlmann, C. Thomsen, A. Löffert, C. Gross, W. Assmus. 2005-08-09. Raman Response of Magnetic Excitations in Cuprate Ladders and Planes. https://doi.org/10.1103/physrevb.72.094419

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

arXiv2026

Point-Group Equivariant Neural Networks for Local Dynamics in Lattice Systems

We develop point-group equivariant neural networks for learning local mappings used in dynamical simulations of lattice systems. The same network acts on a finite neighborhood around each site, respecting lattice translations through shared parameters. The local configuration is decomposed into features that transform according to irreducible representations of the point group, and hidden features retain this organization throughout the network. Equivariant linear maps and symmetry-allowed tensor products then learn nonlinear spatial correlations while preserving the required transformation laws. This approach avoids constructing a fixed set of hand-crafted invariant descriptors, whose selection requires choices about which local correlations to retain. It also allows the complexity of the learned mapping to grow without enlarging its spatial cutoff. We demonstrate the construction by learning the forces governing adiabatic dynamics in the square-lattice Holstein model. Comparisons with exact diagonalization test the accuracy of the predicted forces and the evolution of spatial correlations. Force evaluation scales linearly with system size, allowing the trained model to simulate charge-density-wave ordering on large lattices. These simulations reproduce anomalously slow coarsening of the charge-density-wave domains, illustrating the use of the learned local mapping for collective dynamics.

cond-mat.str-el↗
arXiv2026

Topological Chiral Superconductivity from Doping Correlated Charge Transfer Insulator with Orbital Magnetism

Topological chiral superconductivity has been extensively studied from the perspective of electronic structures in momentum space, while its emergence from real-space processes in strongly interacting systems remains largely unexplored. Here, we study a doped charge-transfer insulator in a strongly repulsive spinless-fermion model with three sublattices and $2π$ flux per unit cell. Combining perturbative analysis, exact diagonalization, and density matrix renormalization group simulations, we establish a topological superconducting ground state with $p+ip$ symmetry. In the large charge-transfer gap limit, chiral charge-transfer excitations generate a correlated-hopping process that provides a microscopic mechanism for electron pairing and its chiral structure. The chiral superconductivity persists into the smaller-gap regime, where chiral excitonic two-particle bound state can emerge. Our results establish a concrete real-space route to topological chiral superconductivity upon doping strongly interacting charge-transfer insulators with orbital magnetism.

cond-mat.str-el↗
arXiv2026

Solving fractional quantum Hall problems with thermodynamic-limit bootstrap

Determining correlated ground states directly in the thermodynamic limit remains a central challenge in quantum many-body physics. Here we develop a quantum many-body bootstrap that yields a rigorous and tight lower bound on the thermodynamic ground-state energy of a fractional quantum Hall system together with an optimized reduced density matrix $ρ_W^\star$ on a spatial window. For sufficiently tight bounds, we find that $ρ_W^\star$ accurately reproduces the ground-state reduced density matrix, as directly tested by its fidelity with known model states. For exactly solvable Laughlin and Moore--Read parent Hamiltonians, the bootstrap also reproduces pair correlations and orbital entanglement spectra (OES). For Landau-level-projected Coulomb interactions across multiple fillings, the energy bounds closely track established thermodynamic estimates, while the window density matrix recovers the familiar $ν=1/3$ Laughlin and $ν=5/2$ Moore--Read states and the composite Fermi liquid at $ν=1/2$. More importantly, the same framework also resolves unsettled regimes. At $ν=1/4$, the OES and real-space correlations identify a composite Fermi liquid, while at $ν=12/5$ the combined diagnostics suggest $\overline{\mathrm{RR}}_3$ as the ground-state order. Our bootstrap therefore provides direct access to both ground-state energies and many-body structure in the thermodynamic limit.

cond-mat.str-el↗