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Raising Bi-O bands above the Fermi energy level of hole-doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ and other cuprate superconductors

Hsin Lin·S. Sahrakorpi·R. S. Markiewicz·A. Bansil
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Abstract

The Fermi surface (FS) of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (Bi2212) predicted by band theory displays Bi-related pockets around the $(π,0)$ point, which have never been observed experimentally. We show that when the effects of hole doping either by substituting Pb for Bi or by adding excess O in Bi2212 are included, the Bi-O bands are lifted above the Fermi energy ($E_F$) and the resulting first-principles FS is in remarkable accord with measurements. With decreasing hole-doping the Bi-O bands drop below $E_F$ and the system self-dopes below a critical hole concentration. Computations on other Bi- as well as Tl- and Hg-based compounds indicate that lifting of the cation-derived band with hole doping is a general property of the electronic structures of the cuprates.

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Hsin Lin, S. Sahrakorpi, R. S. Markiewicz, A. Bansil. 2006-02-03. Raising Bi-O bands above the Fermi energy level of hole-doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ and other cuprate superconductors. https://doi.org/10.1103/physrevlett.96.097001

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