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Ballistic Phonon Thermal Transport in Multi-Walled Carbon Nanotubes

H. -Y. Chiu·V. V. Deshpande·H. W. Ch. Postma·C. N. Lau·C. Mikó·L. Forró·M. Bockrath
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Abstract

We report electrical transport experiments using the phenomenon of electrical breakdown to perform thermometry that probe the thermal properties of individual multi-walled nanotubes. Our results show that nanotubes can readily conduct heat by ballistic phonon propagation, reaching a quantum-mechanical limit to thermal conductance. We determine the thermal conductance quantum, the ultimate limit to thermal conductance for a single phonon channel, and find good agreement with theoretical calculations. Moreover, our results suggest a breakdown mechanism of thermally activated C-C bond breaking coupled with the electrical stress of carrying ~10^12 A/m^2. We also demonstrate a current-driven self-heating technique to improve the conductance of nanotube devices dramatically.

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H. -Y. Chiu, V. V. Deshpande, H. W. Ch. Postma, C. N. Lau, C. Mikó, L. Forró, M. Bockrath. 2005-07-01. Ballistic Phonon Thermal Transport in Multi-Walled Carbon Nanotubes. https://doi.org/10.1103/physrevlett.95.226101

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