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Quantitative analysis of Sr2RuO4 ARPES spectra: Many-body interactions in a model Fermi liquid

N. J. C. Ingle·K. M. Shen·F. Baumberger·W. Meevasana·D. H. Lu·Z. X. Shen·A. Damascelli·S. Nakatsuji·Z. Q. Mao·Y. Maeno·T. Kimura·Y. Tokura
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Abstract

ARPES spectra hold a wealth of information about the many-body interactions in a correlated material. However, the quantitative analysis of ARPES spectra to extract the various coupling parameters in a consistent manner is extremely challenging, even for a model Fermi liquid system. We propose a fitting procedure which allows quantitative access to the intrinsic lineshape, deconvolved of energy and momentum resolution effects, of the correlated 2-dimensional material Sr2RuO4. For the first time in correlated 2-dimensional materials, we find an ARPES linewidth that is narrower than its binding energy, a key property of quasiparticles within Fermi liquid theory. We also find that when the electron-electron scattering component is separated from the electron-phonon and impurity scattering terms it decreases with a functional form compatible with Fermi liquid theory as the Fermi energy is approached. In combination with the previously determined Fermi surface, these results give the first complete picture of a Fermi liquid system via ARPES. Furthermore, we show that the magnitude of the extracted imaginary part of the self-energy is in remarkable agreement with DC transport measurements.

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N. J. C. Ingle, K. M. Shen, F. Baumberger, W. Meevasana, D. H. Lu, Z. X. Shen, A. Damascelli, S. Nakatsuji, Z. Q. Mao, Y. Maeno, T. Kimura, Y. Tokura. 2005-08-04. Quantitative analysis of Sr2RuO4 ARPES spectra: Many-body interactions in a model Fermi liquid. https://doi.org/10.1103/physrevb.72.205114

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