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Hysteresis effects in the phase diagram of multiferroic GdMnO$_3$

J. Baier·D. Meier·K. Berggold·J. Hemberger·A. Balbashov·J. A. Mydosh·T. Lorenz
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Abstract

We present high-resolution thermal expansion $α(T)$ and magnetostriction $ΔL(H)/L$ measurements of GdMnO$_3$, which develops an incommensurate antiferromagnetic order (ICAFM) below $T_{\rm N}\simeq$ 42 K and transforms into a canted A-type antiferromagnet (cAFM) below $T_{\rm c}\simeq 20 $K. In addition, a ferroelectric polarization ${\bf P}||a$ is observed below $T_{\rm FE} $ for finite magnetic fields applied along the $b$ direction. In zero magnetic field we find a strongly anisotropic thermal expansion with certain, rather broad anomalous features. In finite magnetic fields, however, very strong anomalies arise at $T_{\rm c}$ for fields applied along each of the orthorhombic axes and at $T_{\rm FE}$ for fields along the b axis. Both phase transitions are of first-order type and strongly hysteretic. We observe a down-bending of the ICAFM-to-cAFM phase boundary $T_{\rm c}(H)$ for low magnetic fields and our data give evidence for coexisting phases in the low-field low-temperature range.

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J. Baier, D. Meier, K. Berggold, J. Hemberger, A. Balbashov, J. A. Mydosh, T. Lorenz. 2006-03-09. Hysteresis effects in the phase diagram of multiferroic GdMnO$_3$. https://doi.org/10.1103/physrevb.73.100402

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