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Orientation of molecules via laser-induced anti-alignment

E. Gershnabel·I. Sh. Averbukh·R. J. Gordon
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Abstract

We show that field-free molecular orientation induced by a half-cycle pulse may be considerably enhanced by an additional laser pulse inducing molecular anti-alignment. Two qualitatively different enhancement mechanisms are identified depending on the pulse order, and their effects are optimized with the help of quasi-classical as well as fully quantum models.

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E. Gershnabel, I. Sh. Averbukh, R. J. Gordon. 2005-09-14. Orientation of molecules via laser-induced anti-alignment. https://doi.org/10.1103/physreva.73.061401

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