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A. A. Belyanin

Publications and source records attributed to A. A. Belyanin.

14 recordsLinked to original sources

Fermi-Edge Superfluorescence from a Quantum-Degenerate Electron-Hole Gas

We report on the observation of spontaneous bursts of coherent radiation from a quantum-degenerate gas of nonequilibrium electron-hole pairs in semiconductor quantum wells. Unlike typical spontaneous emission from semiconductors, which occurs at the band edge, the observed emission occurs at the quasi-Fermi edge of the carrier distribution. As the carriers are consumed by recombination, the quasi-Fermi energy goes down toward the band edge, and we observe a continuously red-shifting streak. We interpret this emission as cooperative spontaneous recombination of electron-hole pairs, or superfluorescence, which is enhanced by Coulomb interactions near the Fermi edge. This novel many-body enhancement allows the magnitude of the spontaneously developed macroscopic polarization to exceed the maximum value for ordinary superfluorescence, making electron-hole superfluorescence even more "super" than atomic superfluorescence.

cond-mat.mes-hall↗

Review of Anisotropic Terahertz Material Response

Anisotropy is ubiquitous in solids and enhanced in low-dimensional materials. In response to an electromagnetic wave, anisotropic absorptive and refractive properties result in dichroic and birefringent optical phenomena both in the linear and nonlinear optics regimes. Such material properties have led to a diverse array of useful polarization components in the visible and near-infrared, but mature technology is non-existent in the terahertz (THz). Here, we review several novel types of anisotropic material responses observed in the THz frequency range, including both linear and circular anisotropy, which have long-term implications for the development of THz polarization optics. We start with the extreme linear anisotropy of macroscopically aligned carbon nanotubes, arising from their intrinsically anisotropic dynamic conductivity. Magnetically induced anisotropy will then be reviewed, including the giant Faraday effects observed in semiconductors, semimetals, and two-dimensional electron systems.

cond-mat.mtrl-sci↗

Midinfrared Third Harmonic Generation from Macroscopically Aligned Ultralong Single-Wall Carbon Nanotubes

We report the observation of strong third harmonic generation from a macroscopic array of aligned ultralong single-wall carbon nanotubes (SWCNTs) with intense midinfrared radiation. Through power-dependent experiments, we determined the absolute value of the third-order nonlinear optical susceptibility, $χ^{(3)}$, of our SWCNT film to be 5.53 $\times$ 10$^{-12}$ esu, three orders of magnitude larger than that of the fused silica reference we used. Taking account of the filling factor of 8.75% for our SWCNT film, we estimate a $χ^{(3)}$ of 6.32 $\times$ 10$^{-11}$ esu for a fully dense film. Furthermore, through polarization-dependent experiments, we extracted all the nonzero elements of the $χ^{(3)}$ tensor, determining the magnitude of the weaker tensor elements to be $\sim$1/6 of that of the dominant $χ^{(3)}_{zzzz}$ component.

cond-mat.mes-hall↗

Collective Antenna Effects in the Terahertz and Infrared Response of Highly Aligned Carbon Nanotube Arrays

We study macroscopically-aligned single-wall carbon nanotube arrays with uniform lengths via polarization-dependent terahertz and infrared transmission spectroscopy. Polarization anisotropy is extreme at frequencies less than $\sim$3 THz with no sign of attenuation when the polarization is perpendicular to the alignment direction. The attenuation for both parallel and perpendicular polarizations increases with increasing frequency, exhibiting a pronounced and broad peak around 10 THz in the parallel case. We model the electromagnetic response of the sample by taking into account both radiative scattering and absorption losses. We show that our sample acts as an effective antenna due to the high degree of alignment, exhibiting much larger radiative scattering than absorption in the mid/far-infrared range. Our calculated attenuation spectrum clearly shows a non-Drude peak at $\sim$10 THz in agreement with the experiment.

cond-mat.mes-hall↗

Giant Tunable Faraday Effect in a Semiconductor Magneto-plasma for Broadband Terahertz Polarization Optics

We report on a giant Faraday effect in an electron plasma in n-InSb probed via polarization-resolved terahertz (THz) time-domain spectroscopy. Polarization rotation angles and ellipticities reach as large as π/2 and 1, respectively, over a wide frequency range (0.3-2.5 THz) at magnetic fields of a few Tesla. The experimental results together with theoretical simulations show its promising ability to construct broadband and tunable THz polarization optics, such as a circular polarizer, half-wave plate, and polarization modulators.

physics.optics↗

Renormalized Energies of Superfluorescent Bursts from an Electron-Hole Magneto-plasma with High Gain in InGaAs Quantum Wells

We study light emission properties of a population-inverted 2D electron-hole plasma in a quantizing magnetic field. We observe a series of superfluorescent bursts, discrete both in time and energy, corresponding to the cooperative recombination of electron-hole pairs from different Landau levels. The emission energies are strongly renormalized due to many-body interactions among the photogenerated carriers, exhibiting red-shifts as large as 20 meV at 15 T. However, the magnetic field dependence of the lowest Landau level emission line remains excitonic at all magnetic fields. Interestingly, our time-resolved measurements show that this lowest-energy burst occurs only after all upper states become empty, suggesting that this excitonic stability is related to the `hidden symmetry' of 2D magneto-excitons expected in the magnetic quantum limit.

cond-mat.mes-hall↗

Generation of Superfluorescent Bursts from a Fully Tunable Semiconductor Magneto-plasma

Quantum particles sometimes cooperate to develop a macroscopically ordered state with extraordinary properties. Superconductivity and Bose-Einstein condensation are examples of such cooperative phenomena where macroscopic order appears spontaneously. Here, we demonstrate that such an ordered state can also be obtained in an optically excited semiconductor quantum well in a high magnetic field. When we create a dense electron-hole plasma with an intense laser pulse, after a certain delay, an ultrashort burst of coherent radiation emerges. We interpret this striking phenomenon as a manifestation of superfluorescence (SF), in which a macroscopic polarization spontaneously builds up from an initially incoherent ensemble of excited quantum oscillators and then decays abruptly producing giant pulses of coherent radiation. SF has been observed in atomic gases, but the present work represents the first observation of SF in a solid-state setting. While there is an analogy between the recombination of electron-hole pairs and radiative transitions in atoms, there is no a priori reason for SF in semiconductors to be similar to atomic SF. This is a complex many-body system with a variety of ultrafast interactions, where the decoherence rates are at least 1,000 times faster than the radiative decay rate, an unusual situation totally unexplored in previous atomic SF studies. We show, nonetheless, that collective many-body coupling via a common radiation field does develop under certain conditions and leads to SF bursts. The solid-state realization of SF resulted in an unprecedented degree of controllability in the generation of SF, opening up opportunities for both fundamental many-body studies and device applications. We demonstrate that the intensity and delay time of SF bursts are fully tunable through an external magnetic field, temperature, and pump laser power.

cond-mat.mes-hall↗

Giant Superfluorescent Bursts from a Semiconductor Magnetoplasma

Currently, considerable resurgent interest exists in the concept of superradiance (SR), i.e., accelerated relaxation of excited dipoles due to cooperative spontaneous emission, first proposed by Dicke in 1954. Recent authors have discussed SR in diverse contexts, including cavity quantum electrodynamics, quantum phase transitions, and plasmonics. At the heart of these various experiments lies the coherent coupling of constituent particles to each other via their radiation field that cooperatively governs the dynamics of the whole system. In the most exciting form of SR, called superfluorescence (SF), macroscopic coherence spontaneously builds up out of an initially incoherent ensemble of excited dipoles and then decays abruptly. Here, we demonstrate the emergence of this photon-mediated, cooperative, many-body state in a very unlikely system: an ultradense electron-hole plasma in a semiconductor. We observe intense, delayed pulses, or bursts, of coherent radiation from highly photo-excited semiconductor quantum wells with a concomitant sudden decrease in population from total inversion to zero. Unlike previously reported SF in atomic and molecular systems that occur on nanosecond time scales, these intense SF bursts have picosecond pulse-widths and are delayed in time by tens of picoseconds with respect to the excitation pulse. They appear only at sufficiently high excitation powers and magnetic fields and sufficiently low temperatures - where various interactions causing decoherence are suppressed. We present theoretical simulations based on the relaxation and recombination dynamics of ultrahigh-density electron-hole pairs in a quantizing magnetic field, which successfully capture the salient features of the experimental observations.

cond-mat.mes-hall↗

Time-Integrated Evidence for Superfluorescence from Dense Electron-Hole Magneto-Plasmas in Semiconductor Quantum Wells

Cooperative spontaneous recombination (superfluorescence) of electron-hole plasmas in semiconductors has been a challenge to observe due to ultrafast decoherence. We argue that superfluorescence can be achieved in quantum-confined semiconductor systems and present experimental evidence for superfluorescence from high-density photoexcited electron-hole plasmas in quantum wells under high magnetic fields (> 20 T). At a critical magnetic field strength and excitation fluence, we observe a clear transition in the band-edge photoluminescence from omnidirectional output to a randomly directed but highly collimated beam. Changes in the linewidth, carrier density, and magnetic field scaling of the emission spectra correlate precisely with the onset of random directionality and are consistent with cooperative recombination. We further investigate the effects of spot size, temperature, and excitation geometry on the emission properties.

cond-mat.mes-hall↗

Cooperative Recombination of a Quantized High-Density Electron-Hole Plasma

We investigate photoluminescence from a high-density electron-hole plasma in semiconductor quantum wells created via intense femtosecond excitation in a strong perpendicular magnetic field, a fully-quantized and tunable system. At a critical magnetic field strength and excitation fluence, we observe a clear transition in the band-edge photoluminescence from omnidirectional output to a randomly directed but highly collimated beam. In addition, changes in the linewidth, carrier density, and magnetic field scaling of the PL spectral features correlate precisely with the onset of random directionality, indicative of cooperative recombination from a high density population of free carriers in a semiconductor environment.

cond-mat.other↗

Constraints on the Extremely High-Energy Cosmic Ray Accelerators from Classical Electrodynamics

We find the general requirements, set by classical electrodynamics, to the sources of extremely high-energy cosmic rays (EHECRs). It is shown that the parameters of EHECR accelerators are strongly limited not only by the particle confinement in large-scale magnetic field or by the difference in electric potentials (generalized Hillas criterion), but also by the synchrotron radiation, the electro-bremsstrahlung, or the curvature radiation of accelerated particles. Optimization of these requirements in terms of accelerator's size and magnetic field strength results in the ultimate lower limit to the overall source energy, which scales as the fifth power of attainable particle energy. Hard gamma-rays accompanying generation of EHECRs can be used as a probe for potential acceleration sites. We apply the results to several populations of astrophysical objects -- potential EHECR sources -- and discuss their ability to accelerate protons to $10^{20}$ eV and beyond. A possibility to gain from ultrarelativistic bulk flows is emphasized, with Active Galactic Nuclei and Gamma-Ray Bursts being the examples.

astro-ph↗

The influence of free neutrons on dynamics and radiation of astrophysical plasmas

We present arguments in favor of the presence of free neutrons in plasmas generated by compact astrophysical objects and find conditions necessary for the formation of the neutron component. The broad range of phenomena caused by neutrons includes both dynamical (sources' variability, transition of fireballs to the two-flow regime) and kinetic (fission of helium nuclei by neutrons, electromagnetic cascade, emission in annihilation and nuclear lines, neutrino losses) effects. The presented theory can be applied to internal regions of accretion disks, jets in microquasars, and gamma-ray burst (GRB) fireballs.

astro-ph↗

Formation and dynamics of self-sustained neutron haloes in disk accreting sources

It has been recognized long ago that the presence of hot plasma in the inner accretion disks around black holes could lead to the neutron production via dissociation of helium nuclei. We show that, for a broad range of accretion parameters, neutrons effectively decouple from protons and pile up in the inner disk leading to the formation of self-sustained halo. This means that new neutrons in the halo are supplied mainly by the splitting of helium nuclei in their collisions with existing neutrons. Once formed, such a halo can exist even if the proton temperature is much lower than the energy threshold of helium dissociation. We show that neutron haloes can be the natural source of relativistic electrons and positrons, providing characteristic comptonization spectra and hard spectral tails observed in many black hole candidates, and also giving rise to relativistic outflows. Deuterium gamma-ray line at 2.2 MeV resulting from neutron capture is also expected at a level detectable by future INTEGRAL mission. Furthermore, the presence of a neutron halo strongly affects the dynamics of accretion and leads to the rich variety of transient dynamical regimes.

astro-ph↗

Infrared generation in low-dimensional semiconductor heterostructures via quantum coherence

A new scheme for infrared generation without population inversion between subbands in quantum-well and quantum-dot lasers is presented and documented by detailed calculations. The scheme is based on the simultaneous generation at three frequencies: optical lasing at the two interband transitions which take place simultaneously, in the same active region, and serve as the coherent drive for the IR field. This mechanism for frequency down-conversion does not rely upon any ad hoc assumptions of long-lived coherences in the semiconductor active medium. And it should work efficiently at room temperature with injection current pumping. For optimized waveguide and cavity parameters, the intrinsic efficiency of the down-conversion process can reach the limiting quantum value corresponding to one infrared photon per one optical photon. Due to the parametric nature of IR generation, the proposed inversionless scheme is especially promising for long-wavelength (far- infrared) operation.

quant-ph↗